Electrochemical and photochemical CO2 reduction using diamond

被引：30

作者：

Yu, Siyu ^{[1
]}

Yang, Nianjun ^{[2
]}

Liu, Shetian ^{[1
]}

Jiang, Xin ^{[2
]}

机构：

[1] Southwest Univ, Sch Chem & Chem Engn, Chongqing 400715, Peoples R China

[2] Univ Siegen, Inst Mat Engn, D-57076 Siegen, Germany

来源：

CARBON | 2021年 / 175卷 / 175期

基金：

中国国家自然科学基金;

关键词：

Diamond catalysts; Electrochemical CO2 reduction; Photochemical CO2 reduction; CARBON-DIOXIDE; FORMIC-ACID; PHOTOELECTROCHEMICAL REDUCTION; ELECTROCATALYTIC CONVERSION; BORON; ELECTRODES; FORMATE; CATALYSTS; FUELS; WATER;

D O I：

10.1016/j.carbon.2021.01.116

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Catalysts are needed for electrochemical and photochemical reduction of CO2 into valuable chemicals. Diamond and its related materials have been regarded as a promising class of catalysts for CO2 reduction. With varied forms, structures, dopants, sp(2)/sp(3) ratios, surface functionalities, and the combination with different co-catalysts, a great diversity of diamond-based catalysts have been fabricated for CO2 reduction. This review summarizes state-of-art progress and achievements on the electrochemical CO2 reduction using different diamond and related electrodes, along with the selection of electrolytes and applied conditions. The applications of diamond nanoparticles and diamond related films for photochemical CO2 reduction are highlighted. The advanced strategies to further improve the catalytic activity of diamond towards CO2 reduction have been discussed and outlined. (C) 2021 Elsevier Ltd. All rights reserved.

引用

页码：440 / 453

页数：14

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