Solar energy conversion in a photoelectrochemical biofuel cell

被引：54
|
作者：
Hambourger, Michael
Kodis, Gerdenis
Vaughn, Michael D.
Moore, Gary F.
Gust, Devens [1 ]
Moore, Ana L.
Moore, Thomas A.
机构：
[1] Arizona State Univ, Ctr Bioenergy & Photosynth, Tempe, AZ 85287 USA
来源：
DALTON TRANSACTIONS | 2009年 / 45期
关键词：
PHOTOINDUCED ELECTRON-TRANSFER; CHARGE RECOMBINATION KINETICS; HYDROGEN-PRODUCTION; FEFE HYDROGENASE; CLOSTRIDIUM-PASTEURIANUM; SPECTRAL SENSITIZATION; POLYPYRIDYL COMPLEXES; ADENINE-DINUCLEOTIDE; SEMICONDUCTOR-FILMS; PHOTOSYSTEM-II;
D O I：
10.1039/b912170f
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
A photoelectrochemical biofuel cell has been developed which incorporates aspects of both an enzymatic biofuel cell and a dye-sensitized solar cell. Photon absorption at a porphyrin-sensitized n-type semiconductor electrode gives rise to a charge-separated state. Electrons and holes are shuttled to appropriate cathodic and anodic catalysts, respectively, allowing the production of electricity, or a reduced fuel, via the photochemical oxidation of a biomass-derived substrate. The operation of this device is reviewed. The use of alternate anodic redox mediators provides insight regarding loss mechanisms in the device. Design strategies for enhanced performance are discussed.
引用
收藏
页码：9979 / 9989
页数：11
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