On the long-distance charge transport in DNA-like macromolecules

被引:0
|
作者
Chevizovich, D. [1 ]
Chizhov, A., V [2 ,3 ]
Ivic, Z. [1 ]
Reshetnyak, A. A. [4 ]
机构
[1] Univ Belgrade, Vinca Inst Nucl Sci, Lab Theoret & Condensed Matter Phys, POB 522, Belgrade 11001, Serbia
[2] Joint Inst Nucl Res, Lab Radiat Biol, Joliot Curie 6, Dubna 141980, Russia
[3] Dubna State Univ, Univ Skaya 19, Dubna 141980, Russia
[4] Inst Strength Phys & Mat Sci SB RAS, Acad Sky Ave 2-4, Tomsk 634021, Russia
来源
关键词
charge migration; DNA soliton; adiabatic polaron; interchain coupling; POLARON; SOLITONS;
D O I
10.17586/2220-8054-2021-12-1-32-41
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
In this paper, we investigate the possibility of stable migration of charge carriers over long distances in DNA-like macromolecular structures in the form of an adiabatic soliton and derive the conditions for the formation of solitons. We find two types of soliton solutions: symmetric and antisymmetric. Comparing the energy of both types of soliton solutions with the energy of free extra charge, we find the region of the system parameters in which the soliton states are more energetically favorable than the states of quasi-free charges. At the same time, which of the two mentioned soliton solutions corresponds to an energetically favorable state depends on the ratio of the energy parameters of the molecular structure.
引用
收藏
页码:32 / 41
页数:10
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