Incorporation of angular momentum anisotropy into the analysis of resonant four-wave mixing spectroscopy

被引：23
|
作者：
Wasserman, TAW
Vaccaro, PH
Johnson, BR
机构：
[1] YALE UNIV,DEPT CHEM,NEW HAVEN,CT 06520
[2] RICE UNIV,DEPT CHEM,HOUSTON,TX 77251
[3] RICE UNIV,RICE QUANTUM INST,HOUSTON,TX 77251
来源：
JOURNAL OF CHEMICAL PHYSICS | 1997年 / 106卷 / 15期
关键词：
D O I：
10.1063/1.473620
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
A state-multipole expansion of the zero-order density operator has been used to derive analytical signal expressions for near-resonant degenerate four-wave mixing spectroscopy performed on systems that possess angular momentum anisotropy. The predictions of this formalism are found to be in good agreement with experimental optical-optical double resonance measurements involving aligned intermediate states. (C) 1997 American Institute of Physics.
引用
收藏
页码：6314 / 6319
页数：6
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