Polyrotaxane-like and Interpenetrating Metal-Organic Frameworks (MOFs) Constructed from Biphenyl-4,4′-Dicarboxylate and Bis(imidazole) Ligand

被引：59

作者：

Liu, Yang ^{[1
]}

Qi, Yan ^{[1
]}

Lv, Yan-Yan ^{[1
]}

Che, Yun-Xia ^{[1
]}

Zheng, Ji-Min ^{[1
]}

机构：

[1] Nankai Univ, Dept Chem, Tianjin 300071, Peoples R China

来源：

CRYSTAL GROWTH & DESIGN | 2009年 / 9卷 / 11期

基金：

中国国家自然科学基金;

关键词：

CAMBRIDGE STRUCTURAL DATABASE; INORGANIC 3D NETWORKS; COORDINATION POLYMERS; 3-DIMENSIONAL NETWORKS; CRYSTAL-STRUCTURE; HYDROTHERMAL SYNTHESIS; HELICAL CHAINS; CO-LIGANDS; NET; ANIONS;

D O I：

10.1021/cg9006372

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The paper presents three interesting entanglement systems, including two polyrotaxane-like and one interpene-trating frameworks, namely, [Co(L-1)(bpdc)] (1), [Co(L-2)(bpdc)] (2), and [Co(L-3)1.5(bpdc)(H2O)]center dot(L-3) (3), constructed from biphenyl-4,4'-dicarboxylate and bis(imidazole) ligands (L-1 = 1,6-bis(imidazol-1-yl)-hexane, and rods that are interlaced in a parallel fashion to result in 2D -> 2D polyrotaxane-like motifs (L-2 = 1,4-bis(imidazol-1-ylmethyl)benzene and L-3 = 1,4-bis(1-imidazolyl)-benzene)). Both compounds 1 and 2 contain loops. Compound 3 represents the first example of a triply interpenetrated 5-connected 4(4) 6(6) topology network.

引用

页码：4797 / 4801

页数：5

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