Exchange interaction and phonon confinement in CdSe quantum dots

被引:91
|
作者
Woggon, U
Gindele, F
Wind, O
Klingshim, C
机构
[1] Institut für Angewandte Physik der Universität Karlsruhe, 76131 Karlsruhe
来源
PHYSICAL REVIEW B | 1996年 / 54卷 / 03期
关键词
D O I
10.1103/PhysRevB.54.1506
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The fine structure of the lowest (1S(3/2), 1s(e)) electron-hole pair state has been studied for CdSe quantum dots embedded in glass and with sizes R<a(B). Besides the very narrow peaks from the exchange-split lowest pair states (full width at half maximum of 2 meV), two additional structures have been found in luminescence and assigned to confined acoustic photons. The observation of discrete acoustic phonons in the emission spectra verifies the importance of low-frequency acoustic phonons for energy relaxation in quantum dots. The size dependence of the different peaks has been determined and compared with theoretical models.
引用
收藏
页码:1506 / 1509
页数:4
相关论文
共 50 条
  • [41] Electron phonon interaction and polaron effects in quantum dots
    Verzelen, O
    Hameau, S
    Guldner, Y
    Gérard, JM
    Ferreira, R
    Bastard, G
    [J]. JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS SHORT NOTES & REVIEW PAPERS, 2001, 40 (3B): : 1941 - 1946
  • [42] Relaxation of Exciton Confinement in CdSe Quantum Dots by Modification with a Conjugated Dithiocarbamate Ligand
    Frederick, Matthew T.
    Weiss, Emily A.
    [J]. ACS NANO, 2010, 4 (06) : 3195 - 3200
  • [43] Dependency of Wavelength of CdSe, ZnS And GaAs Quantum Dots on Dot Radius: Quantum Confinement Effect
    Kurmendra
    Paul, Madhumita
    Mandal, Dhruba Kr.
    [J]. 2015 INTERNATIONAL CONFERENCE ON ELECTRICAL, ELECTRONICS, SIGNALS, COMMUNICATION AND OPTIMIZATION (EESCO), 2015,
  • [44] State-resolved exciton - Phonon couplings in CdSe semiconductor quantum dots
    Sagar, D. M.
    Cooney, Ryan R.
    Sewall, Samuel L.
    Kambhampati, Patanjali
    [J]. JOURNAL OF PHYSICAL CHEMISTRY C, 2008, 112 (25): : 9124 - 9127
  • [45] Comparison of three empirical force fields for phonon calculations in CdSe quantum dots
    Kelley, Anne Myers
    [J]. JOURNAL OF CHEMICAL PHYSICS, 2016, 144 (21):
  • [46] Electron-Phonon Coupling in CdSe/CdS Core/Shell Quantum Dots
    Lin, Chen
    Gong, Ke
    Kelley, David F.
    Kelley, Anne Myers
    [J]. ACS NANO, 2015, 9 (08) : 8131 - 8141
  • [47] Theoretical Study of Electron-Phonon Relaxation in PbSe and CdSe Quantum Dots: Evidence for Phonon Memory
    Kilina, Svetlana V.
    Kilin, Dmitri S.
    Prezhdo, Victor V.
    Prezhdo, Oleg V.
    [J]. JOURNAL OF PHYSICAL CHEMISTRY C, 2011, 115 (44): : 21641 - 21651
  • [48] Interaction of CdSe/ZnS quantum dots: Among themselves and with matrices
    Liu, K.
    Schmedake, T. A.
    Daneshvar, K.
    Tsu, R.
    [J]. MICROELECTRONICS JOURNAL, 2007, 38 (6-7) : 700 - 705
  • [49] Competition between zero-phonon and phonon-assisted luminescence in colloidal CdSe quantum dots
    Wijnen, F. J. P.
    Blokland, J. H.
    Chin, P. T. K.
    Christianen, P. C. M.
    Maan, J. C.
    [J]. PHYSICAL REVIEW B, 2008, 78 (23)
  • [50] Quantum confinement in CdSe nanocrystallites
    Andersen, KE
    Fong, CY
    Pickett, WE
    [J]. JOURNAL OF NON-CRYSTALLINE SOLIDS, 2002, 299 : 1105 - 1110