We study photoinduced ultrafast coherent oscillations originating from orbital degrees of freedom in the one-dimensional two-orbital Hubbard model. By solving the time-dependent Schrodinger equation for the numerically exact many-electron wave function, we obtain time-dependent optical response functions. The calculated spectra show characteristic coherent oscillations that vary with the frequency of probe light. A simple analysis for the dominant oscillating components clarifies that these photoinduced oscillations are caused by the quantum interference between photogenerated states. The oscillation attributed to the Raman-active orbital excitations (orbitons) clearly appears around the charge-transfer peak.
机构:
Ctr Atom Bariloche, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina
CNEA, Inst Balseiro, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina
Consejo Nacl Invest Cient & Tecn, RA-8400 San Carlos De Bariloche, Rio Negro, ArgentinaCtr Atom Bariloche, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina
Hallberg, K.
Nunez-Fernandez, Y.
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机构:
Ctr Atom Bariloche, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina
CNEA, Inst Balseiro, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina
Consejo Nacl Invest Cient & Tecn, RA-8400 San Carlos De Bariloche, Rio Negro, ArgentinaCtr Atom Bariloche, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina
机构:
Chonbuk Natl Univ, Dept Phys, Jeon Ju 561756, South KoreaChonbuk Natl Univ, Dept Phys, Jeon Ju 561756, South Korea
Munkhbaatar, Purevdorj
Myung-Whun, Kim
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Chonbuk Natl Univ, Dept Phys, Jeon Ju 561756, South Korea
Chonbuk Natl Univ, Inst Photon & Informat Technol, Jeon Ju 561756, South KoreaChonbuk Natl Univ, Dept Phys, Jeon Ju 561756, South Korea