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In situ construction of an SnO2/g-C3N4 heterojunction for enhanced visible-light photocatalytic activity
被引:122
|作者:
Chen, Xi
[1
]
Zhou, Banghong
[1
]
Yang, Shuanglei
[1
]
Wu, Hanshuo
[1
]
Wu, Yuxin
[1
]
Wu, Laidi
[1
]
Pan, Jun
[1
]
Xiong, Xiang
[1
]
机构:
[1] Cent South Univ, State Key Lab Powder Met, Changsha 410083, Hunan, Peoples R China
来源:
基金:
美国国家科学基金会;
关键词:
GRAPHITIC CARBON NITRIDE;
HYDROGEN-PRODUCTION;
OPTICAL-PROPERTIES;
NANOWIRE ARRAYS;
G-C3N4;
DEGRADATION;
TIO2;
PERFORMANCE;
PHOTODEGRADATION;
HETEROSTRUCTURES;
D O I:
10.1039/c5ra11801h
中图分类号:
O6 [化学];
学科分类号:
0703 ;
摘要:
Herein, a strong heterojunction, consisting of SnO2 nanoparticles grown on layered g-C3N4 nanosheets, was rationally designed and successfully synthesized via a facile hydrothermal method. The morphology, chemical structure, optical and electronic properties of the obtained SnO2/g-C3N4 hybrid nanocomposites were characterized. Furthermore, the photocatalytic activity of the novel photocatalysts was assessed. The results clearly indicate that the SnO2/g-CN-72.12% nanocomposite photocatalysts shows a stable cycle performance and exhibits significantly enhanced photocatalytic activity, which is 89 and 17 times higher than those of pure SnO2 and g-C3N4, respectively. The synergistic effect of the SnO2/g-C3N4 heterojunction can effectively accelerate the separation of photo-generated carriers and enhance the efficiency of interfacial charge transfer, which are proposed to be responsible for the enhancement of the photocatalytic activities. This study provides a low-cost and large-scale synthesis route for the production of visible light responsive photocatalysts that have potential in environmental purification applications.
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页码:68953 / 68963
页数:11
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