Synthesis of high-temperature CO2 adsorbents from organo-layered double hydroxides with markedly improved CO2 capture capacity

被引:136
|
作者
Wang, Qiang [1 ]
Tay, Hui Huang [1 ]
Zhong, Ziyi [1 ]
Luo, Jizhong [1 ]
Borgna, Armando [1 ]
机构
[1] ASTAR, ICES, Jurong Isl 627833, Singapore
关键词
HYDROTALCITE-LIKE COMPOUNDS; CARBON-DIOXIDE; STRUCTURAL-CHARACTERIZATION; PROMOTED HYDROTALCITE; HYDROGEN-PRODUCTION; ADSORPTION; SORPTION; NANOCOMPOSITES; OXIDES; DECOMPOSITION;
D O I
10.1039/c2ee21409a
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Synthesis of highly efficient high-temperature CO2 adsorbents from organo-layered double hydroxides (LDHs) is presented for the first time. We demonstrate that the intercalation of long carbon-chain organic anions markedly increases the CO2 capture capacity (1.25 mmol g(-1)), 2.5 times higher than that of traditional adsorbents (0.5 mmol g(-1)). This work suggests a new direction for the synthesis of high-temperature CO2 adsorbents.
引用
收藏
页码:7526 / 7530
页数:5
相关论文
共 50 条
  • [31] Carbonaceous materials as adsorbents for CO2 capture: synthesis and modification
    Gao, Xingyuan
    Yang, Shiting
    Hu, Lifen
    Cai, Shiyi
    Wu, Liqing
    Kawi, Sibudjing
    [J]. CARBON CAPTURE SCIENCE & TECHNOLOGY, 2022, 3
  • [32] Layered double hydroxides for CO2 adsorption at moderate temperatures: Synthesis and amelioration strategies
    Santamaria, L.
    Korili, S. A.
    Gil, A.
    [J]. CHEMICAL ENGINEERING JOURNAL, 2023, 455
  • [33] CO2 EFFECTS AT HIGH-TEMPERATURE
    LAWTON, JH
    [J]. NATURE, 1994, 372 (6507) : 626 - 626
  • [34] High temperature materials for CO2 capture
    Singh, Ranjeet
    Reddy, M. K. Ram
    Wilson, Simon
    Joshi, Kaustubh
    da Costa, Joao C. Diniz
    Webley, Paul
    [J]. GREENHOUSE GAS CONTROL TECHNOLOGIES 9, 2009, 1 (01): : 623 - 630
  • [35] A study on high temperature CO2 capture by improved hydrotalcite sorbents
    Hanif, Aamir
    Dasgupta, Soumen
    Divekar, Swapnil
    Arya, Aarti
    Garg, Madhukar O.
    Nanoti, Anshu
    [J]. CHEMICAL ENGINEERING JOURNAL, 2014, 236 : 91 - 99
  • [36] A study on high temperature CO2 capture by improved hydrotalcite sorbents
    [J]. Nanoti, A. (anshu@iip.res.in), 1600, Elsevier B.V., Netherlands (236):
  • [37] Photocatalytic Conversion of CO2 in Water over Layered Double Hydroxides
    Teramura, Kentaro
    Iguchi, Shoji
    Mizuno, Yuto
    Shishido, Tetsuya
    Tanaka, Tsunehiro
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2012, 51 (32) : 8008 - 8011
  • [38] Selectivity of photoreduction CO2 by tuning the defects in layered double hydroxides
    Li, Jinghong
    [J]. CHINESE SCIENCE BULLETIN-CHINESE, 2019, 64 (31): : 3151 - 3152
  • [39] CO2 adsorption and desorption properties of calcined layered double hydroxides
    Colonna, S.
    Bastianini, M.
    Sisani, M.
    Fina, A.
    [J]. JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY, 2018, 133 (02) : 869 - 879
  • [40] CO2 Capture by Temperature Swing Adsorption: Working Capacity As Affected by Temperature and CO2 Partial Pressure
    Raganati, Federica
    Chirone, Riccardo
    Ammendola, Paola
    [J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2020, 59 (08) : 3593 - 3605