Synthesis of high-temperature CO2 adsorbents from organo-layered double hydroxides with markedly improved CO2 capture capacity

被引:136
|
作者
Wang, Qiang [1 ]
Tay, Hui Huang [1 ]
Zhong, Ziyi [1 ]
Luo, Jizhong [1 ]
Borgna, Armando [1 ]
机构
[1] ASTAR, ICES, Jurong Isl 627833, Singapore
关键词
HYDROTALCITE-LIKE COMPOUNDS; CARBON-DIOXIDE; STRUCTURAL-CHARACTERIZATION; PROMOTED HYDROTALCITE; HYDROGEN-PRODUCTION; ADSORPTION; SORPTION; NANOCOMPOSITES; OXIDES; DECOMPOSITION;
D O I
10.1039/c2ee21409a
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Synthesis of highly efficient high-temperature CO2 adsorbents from organo-layered double hydroxides (LDHs) is presented for the first time. We demonstrate that the intercalation of long carbon-chain organic anions markedly increases the CO2 capture capacity (1.25 mmol g(-1)), 2.5 times higher than that of traditional adsorbents (0.5 mmol g(-1)). This work suggests a new direction for the synthesis of high-temperature CO2 adsorbents.
引用
收藏
页码:7526 / 7530
页数:5
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