An All-in-One Electrode for High-Performance Liquid-Feed Micro Polymer Electrolyte Membrane Fuel Cells

被引:23
|
作者
Li, Yinshi [1 ]
He, Yaling [1 ]
机构
[1] Xi An Jiao Tong Univ, Sch Energy & Power Engn, Key Lab Thermofluid Sci & Engn MOE, Xian 710049, Shaanxi, Peoples R China
关键词
ANION-EXCHANGE MEMBRANE; MASS-TRANSPORT; MODEL;
D O I
10.1149/2.0861607jes
中图分类号
O646 [电化学、电解、磁化学];
学科分类号
081704 ;
摘要
Contrary to the conventional layer-separated electrode design, we report a metal foam-based all-in-one electrode that incorporates the flow field, backing layer, micro-porous layer, and catalyst layer into a whole. This innovative design facilitates the mass and charge transport as well as extends the three-phase boundary, thereby enabling to miniaturize the cell system while enhance the power output. It has been demonstrated that when applying a pair of 4.0 x 4.0 x 0.5 mm (length x width x height) all-in-one electrodes to the liquid-feed micro polymer electrolyte membrane fuel cell, the peak power density goes up to 123 mW cm(-2) even at room temperature, which is much higher than that of the conventional cell system. The present architecture design meets the potential demand of the high-capacity lab-on-a-chip applications. (C) 2016 The Electrochemical Society. All rights reserved.
引用
收藏
页码:F663 / F667
页数:5
相关论文
共 50 条
  • [1] Cross-over and performance modeling of liquid-feed Polymer Electrolyte Membrane Direct Ethanol Fuel Cells
    Suresh, N. S.
    Jayanti, S.
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2011, 36 (22) : 14648 - 14658
  • [2] High-Performance and Durable Membrane Electrode Assemblies for High-Temperature Polymer Electrolyte Membrane Fuel Cells
    Huaneng Su
    Cecil Felix
    Olivia Barron
    Piotr Bujlo
    Bernard J. Bladergroen
    Bruno G. Pollet
    Sivakumar Pasupathi
    [J]. Electrocatalysis, 2014, 5 : 361 - 371
  • [3] High-Performance and Durable Membrane Electrode Assemblies for High-Temperature Polymer Electrolyte Membrane Fuel Cells
    Su, Huaneng
    Felix, Cecil
    Barron, Olivia
    Bujlo, Piotr
    Bladergroen, Bernard J.
    Pollet, Bruno G.
    Pasupathi, Sivakumar
    [J]. ELECTROCATALYSIS, 2014, 5 (04) : 361 - 371
  • [4] Comprehensive one-dimensional, semi-analytical, mathematical model for liquid-feed polymer electrolyte membrane direct methanol fuel cells
    Kareemulla, D.
    Jayanti, S.
    [J]. JOURNAL OF POWER SOURCES, 2009, 188 (02) : 367 - 378
  • [5] Comparison of ethanol and methanol oxidation in a liquid-feed solid polymer electrolyte fuel cell at high temperature
    Aricò, AS
    Cretì, P
    Antonucci, PL
    Antonucci, V
    [J]. ELECTROCHEMICAL AND SOLID STATE LETTERS, 1998, 1 (02) : 66 - 68
  • [6] The design and construction of high-performance direct methanol fuel cells. 1. Liquid-feed systems
    Hogarth, M
    Christensen, P
    Hamnett, A
    Shukla, A
    [J]. JOURNAL OF POWER SOURCES, 1997, 69 (1-2) : 113 - 124
  • [7] High-performance membrane-electrode assembly with an optimal polytetrafluoroethylene content for high-temperature polymer electrolyte membrane fuel cells
    Jeong, Gisu
    Kim, MinJoong
    Han, Junyoung
    Kim, Hyoung-Juhn
    Shul, Yong-Gun
    Cho, EunAe
    [J]. JOURNAL OF POWER SOURCES, 2016, 323 : 142 - 146
  • [8] Performance of dimethoxymethane and trimethoxymethane in liquid-feed direct oxidation fuel cells
    Prakash, G. K. S.
    Smart, M. C.
    Olah, G. A.
    Narayanan, S. R.
    Chun, W.
    Surampudi, S.
    Halpert, G.
    [J]. JOURNAL OF POWER SOURCES, 2007, 173 (01) : 102 - 109
  • [9] Effect of methanol crossover in a liquid-feed polymer-electrolyte direct methanol fuel cell
    Ravikumar, MK
    Shukla, AK
    [J]. JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1996, 143 (08) : 2601 - 2606
  • [10] High-Performance Fuel Cells with a Plasma-Etched Polymer Electrolyte Membrane with Microhole Arrays
    Seol, Changwook
    Jang, Segeun
    Lee, Jinwon
    Le Vu Nam
    Tuyet Anh Pham
    Koo, Seunghoe
    Kim, Kyeongtae
    Jang, Jue-Hyuk
    Kim, Sang Moon
    Yoo, Sung Jong
    [J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING, 2021, 9 (17): : 5884 - 5894