Using the Near-Field Coupling of a Sharp Tip to Tune Fluorescence-Emission Fluctuations during Quantum-Dot Blinking

被引：21

作者：

Shafran, Eyal ^{[1
]}

Mangum, Benjamin D. ^{[1
]}

Gerton, Jordan M. ^{[1
]}

机构：

[1] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA

来源：

PHYSICAL REVIEW LETTERS | 2011年 / 107卷 / 03期

基金：

美国国家科学基金会;

关键词：

SCANNING OPTICAL MICROSCOPY; SINGLE-MOLECULE; SEMICONDUCTOR NANOCRYSTALS; CARBON NANOTUBE; ENERGY-TRANSFER; INTENSITY; ANTENNAS; STATES;

D O I：

10.1103/PhysRevLett.107.037403

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

We demonstrate that the cycling between internal states of quantum dots during fluorescence blinking can be used to tune the near-field coupling with a sharp tip. In particular, the fluorescence emission from states with high quantum yield is quenched due to energy transfer, while that from low-yield states is elevated due to field enhancement. Thus, as a quantum dot blinks, its emission fluctuations are progressively suppressed upon approach of a tip.

引用

页数：4

共 38 条

[31] Efficient Emission Enhancement of Single CdSe/CdS/PMMA Quantum Dots through Controlled Near-Field Coupling to Plasmonic Bullseye Resonators
Werschler, F.
Lindner, B.
Hinz, C.
Conradt, F.
Gumbsheimer, P.
Behovits, Y.
Negele, C.
de Roo, T.
Tzang, O.
Mecking, S.
Leitenstorfer, A.
Seletskiy, D. V.
NANO LETTERS, 2018, 18 (09) : 5396 - 5400
[32] Imaging Intermolecular Exciton Coupling in Metal-Free Phthalocyanine Nanofilms Using Tip-Enhanced Near-Field Optical Microscopy
Hermann, R.
Gordon, M. J.
JOURNAL OF PHYSICAL CHEMISTRY C, 2018, 122 (26): : 14796 - 14804
[33] Homogeneous linewidth study of a single In0.5Ga0.5As quantum dot at high temperature by using near-field scanning optical microscope
Matsuda, Kazunari, 2000, IEEE, Piscataway, NJ, United States
[34] Time-resolved emission from self-assembled single quantum dots using scanning near-field optical microscope
Ono, M
Matsuda, K
Saiki, T
Nishi, K
Mukaiyama, T
Kuwata-Gonokami, M
JAPANESE JOURNAL OF APPLIED PHYSICS PART 2-LETTERS, 1999, 38 (12A): : L1460 - L1462
[35] Determination of the Spatial Resolution of an Aperture-type Near-field Scanning Optical Microscope Using a Standard Sample of a Quantum-dot-embedded Polymer Film
Kim, Jeongyong
Kim, D. C.
Nakajima, K.
Mitsui, T.
Aoki, H.
JOURNAL OF THE KOREAN PHYSICAL SOCIETY, 2010, 56 (06) : 1748 - 1753
[36] Using multi-polar scattering and near-field plasmonic resonances to achieve optimal emission enhancement from quantum emitters embedded in dielectric pillars
Inam, Faraz Ahmed
Castelletto, Stefania
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 2021, 38 (12) : 3697 - 3704
[37] A Fusion-Spliced Near-Field Optical Fiber Probe Using Photonic Crystal Fiber for Nanoscale Thermometry Based on Fluorescence-Lifetime Measurement of Quantum Dots
Fujii, Takuro
Taguchi, Yoshihiro
Saiki, Toshiharu
Nagasaka, Yuji
SENSORS, 2011, 11 (09): : 8358 - 8369
[38] Homogeneous linewidth broadening in a In0.5Ga0.5As/GaAs single quantum dot at room temperature investigated using a highly sensitive near-field scanning optical microscope -: art. no. 121304
Matsuda, K
Ikeda, K
Saiki, T
Tsuchiya, H
Saito, H
Nishi, K
PHYSICAL REVIEW B, 2001, 63 (12)

← 1 2 3 4 →