K-edge x-ray-absorption spectroscopy of laser-generated Kr+ and Kr2+

被引:25
|
作者
Southworth, S. H. [1 ]
Arms, D. A. [1 ]
Dufresne, E. M. [1 ]
Dunford, R. W. [1 ]
Ederer, D. L. [1 ]
Hoehr, C. [1 ]
Kanter, E. P. [1 ]
Kraessig, B. [1 ]
Landahl, E. C. [1 ]
Peterson, E. R. [1 ]
Rudati, J. [1 ]
Santra, R. [1 ]
Walko, D. A. [1 ]
Young, L. [1 ]
机构
[1] Argonne Natl Lab, Argonne, IL 60439 USA
来源
PHYSICAL REVIEW A | 2007年 / 76卷 / 04期
关键词
D O I
10.1103/PhysRevA.76.043421
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Tunable, polarized, microfocused x-ray pulses were used to record x-ray absorption spectra across the K edges of Kr+ and Kr2+ produced by laser ionization of Kr. Prominent 1s -> 4p and 5p excitations are observed below the 1s ionization thresholds in accord with calculated transition energies and probabilities. Due to alignment of 4p hole states in the laser-ionization process, the Kr+ 1s -> 4p cross section varies with respect to the angle between the laser and x-ray polarization vectors. This effect is used to determine the Kr+ 4p(3/2) and 4p(1/2) quantum state populations, and these are compared with results of an adiabatic strong-field ionization theory that includes spin-orbit coupling.
引用
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页数:9
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