CO2 bubble behaviors and two-phase flow characteristics in single-serpentine sinusoidal corrugated channels of direct methanol fuel cell

被引:23
|
作者
Su, Xiaoqing [1 ]
Yuan, Wei [1 ]
Lu, Biaowu [1 ]
Zheng, Tianxiang [1 ]
Ke, Yuzhi [1 ]
Zhuang, Ziyi [1 ]
Zhao, Yonghao [1 ]
Tang, Yong [1 ]
Zhang, Shiwei [1 ,2 ]
机构
[1] South China Univ Technol, Sch Mech & Automot Engn, Guangzhou 510640, Guangdong, Peoples R China
[2] City Univ Hong Kong, Dept Mech Engn, Kowloon, Hong Kong, Peoples R China
基金
中国国家自然科学基金;
关键词
Direct methanol fuel cell; Two-phase flow; CO2; bubbles; Sinusoidal corrugated channel; Disturbance structure; Phase field; INTERFACIAL DYNAMICS; REACTANT TRANSPORT; MICROSCALE FLOW; FIELD DESIGNS; PERFORMANCE; ANODE; WATER; DMFC; FLUIDS; VISUALIZATION;
D O I
10.1016/j.jpowsour.2019.227621
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Management of the produced carbon dioxide (CO2) is important to improve the performance of a liquid-feed direct methanol fuel cell (DMFC). This work investigates the CO2 bubble behaviors and the two-phase flow characteristics, using a single sinusoidal corrugated channel as the anode flow field. The magnitude and gradient of the fluid velocity in this channel is higher than the traditional straight pattern, as proven by tracking CO2 bubbles. The use of high magnitude and gradient of velocity enhances CO2 emission and fuel delivery, as well as increases the pressure drop. The vortices in the disturbance structure of the corrugated channel help uniformly deliver the reactants and separate bubbles away from the channel wall. Using excessive values of amplitude A and angular frequency W in the corrugated channel causes serious bubble deformation and extra energy consumption. The effect of disturbance structure is negligible with small values of these two parameters. The cell with a corrugated channel shows a higher performance at different feed rates and concentrations of the methanol fuel. The optimal value of A and W are respectively 0.1and 5. The visualization tests demonstrate that the appearance of CO2 bubbles in the corrugated channel is consistent with the simulation results.
引用
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页数:13
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