A tridentate Ni pincer for aqueous electrocatalytic hydrogen production

被引：77

作者：

Luca, Oana R. ^{[1
]}

Konezny, Steven J. ^{[1
]}

Blakemore, James D. ^{[1
]}

Colosi, Dominic M. ^{[2
]}

Saha, Shubhro ^{[1
]}

Brudvig, Gary W. ^{[1
]}

Batista, Victor S. ^{[1
]}

Crabtree, Robert H. ^{[1
]}

机构：

[1] Yale Univ, Dept Chem, New Haven, CT 06520 USA

[2] Yale Univ, Dept Geol & Geophys, Earth Syst Ctr Stable Isotop Studies, New Haven, CT 06511 USA

来源：

NEW JOURNAL OF CHEMISTRY | 2012年 / 36卷 / 05期

关键词：

COUPLED ELECTRON-TRANSFER; FUNCTIONAL MODELS; COBALT; COMPLEXES; EVOLUTION; REDUCTION; WATER; ELECTROCHEMISTRY; PROTONS; CYCLOADDITION;

D O I：

10.1039/c2nj20912h

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

A Ni-II complex with a redox-active pincer ligand reduces protons at a low overpotential in aqueous acidic conditions. A combined experimental and computational study provides mechanistic insights into a putative catalytic cycle.

引用

页码：1149 / 1152

页数：4

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