Mercury emissions of a coal-fired power plant in Germany

被引：12

作者：

Weigelt, Andreas ^{[1
,6
]}

Slemr, Franz ^{[2
]}

Ebinghaus, Ralf ^{[1
]}

Pirrone, Nicola ^{[3
]}

Bieser, Johannes ^{[1
,4
]}

Boedewadt, Jan ^{[1
]}

Esposito, Giulio ^{[3
]}

van Velthoven, Peter F. J. ^{[5
]}

机构：

[1] HZG, Inst Coastal Res, Geesthacht, Germany

[2] MPI C, Dept Atmospher Chem, Mainz, Germany

[3] CNR, Inst Atmospher Pollut Res, Arcavacata Di Rende, Italy

[4] Deutsch Zentrum Luft & Raumfahrt DLR, Inst Atmospher Phys, Oberpfaffenhofen, Germany

[5] Royal Netherlands Meteorol Inst KNMI, Chem & Climate Div, De Bilt, Netherlands

[6] Fed Maritime & Hydrog Agcy BSH, Hamburg, Germany

来源：

ATMOSPHERIC CHEMISTRY AND PHYSICS | 2016年 / 16卷 / 21期

关键词：

FLUE-GAS DESULFURIZATION; ATMOSPHERIC MERCURY; OXIDIZED MERCURY; UPPER TROPOSPHERE; GASEOUS MERCURY; MODELING MERCURY; SPECIATION; METHYLMERCURY; COMBUSTION; DENUDERS;

D O I：

10.5194/acp-16-13653-2016

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

Hg / SO2, Hg / CO, NOx / SO2 (NOx being the sum of NO and NO2) emission ratios (ERs) in the plume of the coal-fired power plant (CFPP), Lippendorf, near Leipzig, Germany, were determined within the European Tropospheric Mercury Experiment (ETMEP) aircraft campaign in August 2013. The gaseous oxidized mercury (GOM) fraction of mercury emissions was also assessed. Measured Hg / SO2 and Hg / CO ERs were within the measurement uncertainties consistent with the ratios calculated from annual emissions in 2013 reported by the CFPP operator, while the NOx / SO2 ER was somewhat lower. The GOM fraction of total mercury emissions, estimated using three independent methods, was below similar to 25 %. This result is consistent with other findings and suggests that GOM fractions of similar to 40% of CFPP mercury emissions in current emission inventories are overestimated.

引用

页码：13653 / 13668

页数：16

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