Highly Controllable Etchless Perovskite Microlasers Based on Bound States in the Continuum

被引:73
|
作者
Wang, Yuhan [1 ]
Fan, Yubin [1 ]
Zhang, Xudong [1 ]
Tang, Haijun [1 ]
Song, Qinghai [1 ,3 ]
Han, Jiecai [4 ]
Xiao, Shumin [1 ,2 ,3 ]
机构
[1] Harbin Inst Technol, Shenzhen Grad Sch, Minist Ind & Informat Technol, Key Lab Micronano Optoelect Informat Syst, Shenzhen 518055, Peoples R China
[2] Harbin Inst Technol, Natl Key Lab Sci & Technol Adv Composites Special, Shenzhen 518055, Peoples R China
[3] Shanxi Univ, Collaborat Innovat Ctr Extreme Opt, Taiyuan 030006, Shanxi, Peoples R China
[4] Harbin Inst Technol, Natl Key Lab Sci & Technol Adv Composites Special, Harbin 150080, Peoples R China
基金
中国国家自然科学基金;
关键词
bound states in the continuum; etchless grating; perovskite microlasers; polarization vortex; well-controlled laser; NANOWIRE LASERS; VORTEX;
D O I
10.1021/acsnano.1c00673
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Lead halide perovskites have been promising materials for lasing applications. Despite that a series of perovskite microlasers have been reported, their lasing modes are confined by either the as-grown morphology or the etched boundary. The first one is quite random and incompatible with integration, whereas the latter one strongly spoils the laser performances. Herein, we propose and experimentally demonstrate a robust and generic mechanism to realize well-controlled perovskite microlasers without the etching process. By patterning a one-dimensional polymer grating onto a perovskite film, we show that the symmetry-protected bound states in the continuum (BICs) can be formed in it. The intriguing properties of BICs including a widely spread mode profile and high Q factor, associated with the exceptional gain of perovskite, produce single-mode microlasers with high repeatability, controllability, directionality, and a polarization vortex. This mechanism can also be extended to two-dimensional nanostructures, enabling BIC lasers with different topological charges.
引用
收藏
页码:7386 / 7391
页数:6
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