Ladder-like metal diphosphonates exhibiting field-induced magnetic transitions

被引：17
|
作者：
Zhang, Zai-Chao [1 ]
Bao, Song-Song [1 ]
Zheng, Li-Min [1 ]
机构：
[1] Nanjing Univ, Sch Chem & Chem Engn, Inst Coordinat Chem, State Key Lab Coordinat Chem, Nanjing 210093, Peoples R China
来源：
INORGANIC CHEMISTRY COMMUNICATIONS | 2007年 / 10卷 / 09期
基金：
中国国家自然科学基金;
关键词：
manganese; cobalt; diphosphonate; magnetic property; chain structure; spin ladder;
D O I：
10.1016/j.inoche.2007.05.028
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
Two new isomorphous phosphonates M(ahbdpH(2)) center dot H2O [M = Mn (1), Co (2); ahbdpH(4) = 4-amino-1-hydroxybutane-1, 1-diphosphonic acid, C4H13NO7P2] have been hydrotherinally synthesized. Both exhibit a ladder-like chain structure in which the edge-shared {MO6} octahedra are linked by {CPO3} tetrahedra through corner-sharing. The double chains are connected through extensive hydrogen bonds among amino groups, phosphonate oxygen atoms and lattice water molecules, hence generating a three-dimensional network. Magnetic measurements reveal that both experience field-induced magnetic transitions at low temperature. (c) 2007 Elsevier B.V. All rights reserved.
引用
收藏
页码：1063 / 1066
页数：4
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