Facile Preparation of Three-Dimensional MoS2 Aerogels for Highly Efficient Solar Desalination

被引:59
|
作者
Wang, Qingmiao [1 ,3 ]
Guo, Qijing [2 ]
Jia, Feifei [1 ,2 ]
Li, Yanmei [3 ]
Song, Shaoxian [1 ,2 ]
机构
[1] Wuhan Univ Technol, Hubei Key Lab Mineral Resources Proc & Environm, Wuhan 430070, Hubei, Peoples R China
[2] Wuhan Univ Technol, Sch Resources & Environm Engn, Wuhan 430070, Hubei, Peoples R China
[3] Univ Guanajuato, Dept Mines Met & Geol Engn, Guanajuato 36000, Mexico
基金
中国国家自然科学基金;
关键词
functionalized MoS2 nanosheets; 3D MoS2 aerogels; mechanical stability; solar-to-heat conversion; highly efficient solar desalination; MOLYBDENUM-DISULFIDE; HYBRID AEROGELS; POLYDOPAMINE; REMOVAL; NANOPARTICLES; NANOSHEETS; PB2+; DYES;
D O I
10.1021/acsami.0c07162
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Aerogels, with porous channels for water supply and vapor escape, can provide many inherent advantages in solar desalination and wastewater treatment. For the first time, this work demonstrates the preparation of a novel three-dimensional (3D) MoS2 -based aerogel with high porosity and mechanical stability by a facile strategy for solar desalination. This 3D MoS2 aerogel has an excellent light-absorbing efficiency of over 95% within the whole solar spectrum range, enabling a high evaporation efficiency of 88.0% under a low solar irradiation of 1.0 kW m(-2) and superhigh evaporation efficiencies of over 90% under a slightly enhanced solar irradiation of 1.5-3.0 kW m(-2) as well as a remarkable desalination performance. In addition, the excellent mechanical stability of this MoS2 aerogel renders it to be reused for at least 10 cycles with stable water productivity. Because of its 3D architectures with high porosity and easy separation, this MoS2-based aerogel also provides promising applications in solar-driven water purification, sterilization, and so forth.
引用
收藏
页码:32673 / 32680
页数:8
相关论文
共 50 条
  • [41] Facile preparation of a polysilsesquioxane sheet with a three-dimensional structure
    Li, Meng
    Hao, Bin
    Zhang, Linsheng
    Li, Hui
    Lv, Peng
    Yue, Xiu
    Yasin, Akram
    Ma, Peng-Cheng
    MATERIALS CHEMISTRY FRONTIERS, 2021, 5 (19) : 7176 - 7183
  • [42] Three-dimensional Au-decorated MoS2/TiO2 nanomaterials gas sensors for efficient NO2 sensing
    Zhao, Juan
    Zhang, Shurong
    Xu, Mingyu
    Xu, Peiqi
    Wang, Jin
    Gao, Bo
    Materials Science and Engineering: B, 2025, 312
  • [43] Construction of three-dimensional aerogels from electrospun cellulose fibers as highly efficient and reusable oil absorbents
    Zhang, Yirong
    Wang, Yixiang
    SEPARATION AND PURIFICATION TECHNOLOGY, 2025, 353
  • [44] A facile sonochemical route for the synthesis of MoS2/Pd composites for highly efficient oxygen reduction reaction
    Zuo, Ling-Xia
    Jiang, Li-Ping
    Zhu, Jun-Jie
    ULTRASONICS SONOCHEMISTRY, 2017, 35 : 681 - 688
  • [45] Double-layered montmorillonite/MoS2 aerogel with vertical channel for efficient and stable solar interfacial desalination
    Guo, Qijing
    An, Qing
    Yi, Hao
    Jia, Feifei
    Song, Shaoxian
    APPLIED CLAY SCIENCE, 2022, 217
  • [46] Strain-reduced and Photoluminescence Enhanced of MoS2 Emitters on Three-Dimensional Substrate
    Lee, Andrew Boyi
    Chang, Chiao-Yun
    Lin, Hsiang-Ting
    Lai, Ming-Sheng
    Yu, Cheng-Li
    Wu, Chong-Rong
    Chou, He-Chun
    Lin, Shih-Yen
    Chen, Chi
    Shih, Min-Hsiung
    2D PHOTONIC MATERIALS AND DEVICES III, 2020, 11282
  • [47] Three-Dimensional Interconnected Network Architecture with Homogeneously Dispersed Carbon Nanotubes and Layered MoS2 as a Highly Efficient Cathode Catalyst for Lithium-Oxygen Battery
    Hu, Anjun
    Long, Jianping
    Shu, Chaozhu
    Liang, Ranxi
    Li, Jiabao
    ACS APPLIED MATERIALS & INTERFACES, 2018, 10 (40) : 34077 - 34086
  • [48] Three-dimensional MoS2/rGO nanocomposites with homogeneous network structure for supercapacitor electrodes
    Bao, Jun
    Zeng, Xiao-Fei
    Huang, Xie-Jun
    Chent, Ri-Kui
    Wang, Jie-Xin
    Zhang, Liang-Liang
    Chen, Jian-Feng
    JOURNAL OF MATERIALS SCIENCE, 2019, 54 (24) : 14845 - 14858
  • [49] Fabrication of three-dimensional MoS2 -graphene hybrid monoliths and their catalytic performance for hydrodesulfurization
    Wang Xu-zhen
    Liu Ning
    Ho Han
    Wang Xin-ping
    Qiu Jie-shan
    NEW CARBON MATERIALS, 2014, 29 (02) : 81 - 88
  • [50] MoS2 nanosheets assembling three-dimensional nanospheres for enhanced-performance supercapacitor
    Gao, Yong-Ping
    Huang, Ke-Jing
    Wu, Xu
    Hou, Zhi-Qiang
    Liu, Yuan-Yuan
    JOURNAL OF ALLOYS AND COMPOUNDS, 2018, 741 : 174 - 181