Facile Preparation of Three-Dimensional MoS2 Aerogels for Highly Efficient Solar Desalination

被引:59
|
作者
Wang, Qingmiao [1 ,3 ]
Guo, Qijing [2 ]
Jia, Feifei [1 ,2 ]
Li, Yanmei [3 ]
Song, Shaoxian [1 ,2 ]
机构
[1] Wuhan Univ Technol, Hubei Key Lab Mineral Resources Proc & Environm, Wuhan 430070, Hubei, Peoples R China
[2] Wuhan Univ Technol, Sch Resources & Environm Engn, Wuhan 430070, Hubei, Peoples R China
[3] Univ Guanajuato, Dept Mines Met & Geol Engn, Guanajuato 36000, Mexico
基金
中国国家自然科学基金;
关键词
functionalized MoS2 nanosheets; 3D MoS2 aerogels; mechanical stability; solar-to-heat conversion; highly efficient solar desalination; MOLYBDENUM-DISULFIDE; HYBRID AEROGELS; POLYDOPAMINE; REMOVAL; NANOPARTICLES; NANOSHEETS; PB2+; DYES;
D O I
10.1021/acsami.0c07162
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Aerogels, with porous channels for water supply and vapor escape, can provide many inherent advantages in solar desalination and wastewater treatment. For the first time, this work demonstrates the preparation of a novel three-dimensional (3D) MoS2 -based aerogel with high porosity and mechanical stability by a facile strategy for solar desalination. This 3D MoS2 aerogel has an excellent light-absorbing efficiency of over 95% within the whole solar spectrum range, enabling a high evaporation efficiency of 88.0% under a low solar irradiation of 1.0 kW m(-2) and superhigh evaporation efficiencies of over 90% under a slightly enhanced solar irradiation of 1.5-3.0 kW m(-2) as well as a remarkable desalination performance. In addition, the excellent mechanical stability of this MoS2 aerogel renders it to be reused for at least 10 cycles with stable water productivity. Because of its 3D architectures with high porosity and easy separation, this MoS2-based aerogel also provides promising applications in solar-driven water purification, sterilization, and so forth.
引用
收藏
页码:32673 / 32680
页数:8
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