Nitro Lignin-Derived Nitrogen-Doped Carbon as an Efficient and Sustainable Electrocatalyst for Oxygen Reduction

被引：154

作者：

Graglia, Micaela ^{[1
]}

Pampel, Jonas ^{[1
]}

Hantke, Tina ^{[1
]}

Fellinger, Tim-Patrick ^{[1
]}

Esposito, Davide ^{[1
]}

机构：

[1] Max Planck Inst Colloids & Interfaces, D-14424 Potsdam, Germany

来源：

ACS NANO | 2016年 / 10卷 / 04期

关键词：

electrocatalysis; lignin; nitration; nitrogen-doped carbon; ionothermal carbonization; MESOPOROUS CARBONS; POROUS CARBONS; BIOMASS; NITRATION; VALORIZATION; PERFORMANCE;

D O I：

10.1021/acsnano.5b08040

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The use of lignin as a precursor for the synthesis of materials is nowadays considered very interesting from a sustainability standpoint. Here we illustrate the synthesis of a micro-, meso-, and macroporous nitrogen-doped carbon (NDC) using lignin extracted from beech wood via alkaline hydrothermal treatment and successively functionalized via aromatic nitration. The so obtained material is thus carbonized in the eutectic salt melt KCl/ZnCl2. The final NDC shows an excellent activity as electrocatalyst for the oxygen reduction reaction.

引用

页码：4364 / 4371

页数：8

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