Low-moment magnetism in the double perovskites Ba2MOsO6 (M = Li, Na)

被引:36
|
作者
Steele, Andrew J. [1 ]
Baker, Peter J. [2 ]
Lancaster, Tom [1 ]
Pratt, Francis L. [2 ]
Franke, Isabel [1 ]
Ghannadzadeh, Saman [1 ]
Goddard, Paul A. [1 ]
Hayes, William [1 ]
Prabhakaran, D. [1 ]
Blundell, Stephen J. [1 ]
机构
[1] Univ Oxford, Dept Phys, Clarendon Lab, Oxford OX1 3PU, England
[2] Rutherford Appleton Lab, ISIS Pulsed Neutron & Muon Source, Sci & Technol Facil Council, Didcot OX11 0QX, Oxon, England
来源
PHYSICAL REVIEW B | 2011年 / 84卷 / 14期
基金
英国工程与自然科学研究理事会;
关键词
CRYSTAL-GROWTH; OSMIUM;
D O I
10.1103/PhysRevB.84.144416
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The magnetic ground states of the isostructural double perovskites Ba2NaOsO6 and Ba2LiOsO6 are investigated with muon-spin relaxation. In Ba2NaOsO6 long-range magnetic order is detected via the onset of a spontaneous muon-spin precession signal below T-c = 7.2 +/- 0.2 K, while in Ba2LiOsO6 a static but spatially disordered internal field is found below 8 K. A probabilistic argument is used to show from the observed precession frequencies that the magnetic ground state in Ba2NaOsO6 is most likely to be low-moment (approximate to 0.2 mu(B)) ferromagnetism and not canted antiferromagnetism. Ba2LiOsO6 is antiferromagnetic and we find a spin-flop transition at 5.5 T. A reduced osmium moment is common to both compounds, probably arising from a combination of spin-orbit coupling and frustration.
引用
收藏
页数:4
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