Second-order nonlinearities of lead borate glasses poled with different electrodes

被引：2
|
作者：
Ye, Xiaowei [1 ]
Liu, Liying [1 ]
Xu, Lei [1 ]
Wang, Wencheng [1 ]
Affatigato, Mario [2 ]
Feller, Steve [2 ]
机构：
[1] Fudan Univ, Dept Opt Sci & Engn, State Key Lab Adv Photon Mat & Devices, Sch Informat Sci & Engn, Shanghai 200433, Peoples R China
[2] Coe Coll, Dept Phys, Cedar Rapids, IA 52402 USA
来源：
JOURNAL OF NON-CRYSTALLINE SOLIDS | 2008年 / 354卷 / 12-13期
基金：
中国国家自然科学基金; 美国国家科学基金会;
关键词：
nonlinear optics; borates;
D O I：
10.1016/j.jnoncrysol.2006.12.129
中图分类号：
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号：
0805 ; 080502 ;
摘要：
The second-order nonlinearities in thermally poled lead borate glasses were studied. After poling with different electrodes, both bulk and near surface second-order nonlinearities were obtained. The second harmonic generation signal from near surface effect was two orders of magnitude larger than the bulk effect. By simulating the poling process with a multiple carrier model, we concluded that the bulk second-order nonlinearity was caused by the deficiency of Pb2+ in a thick layer after poling, and the near surface second-order nonlinearity was caused by the depletion of H+ in a thin layer when H+ injection from the atmosphere was blocked. (c) 2007 Elsevier B.V. All rights reserved.
引用
收藏
页码：1250 / 1255
页数：6
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