Contamination, ecological and health risks of trace elements in soil of landfill and geothermal sites in Tibet

被引:70
|
作者
Wang, Xutong [1 ]
Dan, Zeng [1 ,2 ]
Cui, Xiaoqiang [1 ]
Zhang, Ruixue [1 ]
Zhou, Shengquan [1 ]
Wenga, Terrence [1 ]
Yan, Beibei [1 ,3 ,4 ]
Chen, Guanyi [2 ]
Zhang, Qiangying [1 ,2 ]
Zhong, Lei [1 ]
机构
[1] Tianjin Univ, Sch Environm Sci & Engn, Tianjin 300072, Peoples R China
[2] Tibet Univ, Sch Sci, Lhasa 850012, Tibet Autonomou, Peoples R China
[3] Tianjin Engn Res Ctr Biomass Derived Gas Oil, Tianjin 300072, Peoples R China
[4] Tianjin Key Lab Biomass Wastes Utilizat, Tianjin 300350, Peoples R China
关键词
Tibet; Soil contamination; Trace element; Ecological risk; Landfill; HEAVY-METAL POLLUTION; SPATIAL-DISTRIBUTION; SOURCE APPORTIONMENT; AGRICULTURAL SOIL; IDENTIFICATION; AREA; VANADIUM; PLATEAU; SPRINGS; EUROPE;
D O I
10.1016/j.scitotenv.2020.136639
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Due to the utilization of landfill technology and geothermal energy production in Tibet, the contamination of the soils and underground water by trace element has currently become a serious problem, both ecologically and to the human health point of view. However, relevant studies concerning this critical problem, particularly in the Tibet area has not been found. Therefore, this study investigated the soil contamination and the spatial distribution of the trace elements in the areas surrounding the Tibetan landfill sites (LS) and geothermal sites (GS) through several pollution evaluation models. In addition, the possible sources of trace elements and their potential impact on public health were also investigated. Results showed that the trace elements in soils nearby LS and GS had moderate to high contamination risk. In soils surrounding LS, mercury had the highest concentration of 0.015 mg/kg and was 6 times higher than the background value of 0.008 mg/kg while in GS, arsenic had the highest concentration of 66.55 mg/kg, and exceeded the soil contamination risk value of 25 mg/kg. Maizhokunggar IS was the most polluted site with an average pollution load index value of 2.95 compared to Naqu, Nyingchi, Shigatse, and Lhasa. 42% of LS were with considerable ecological risk, and all GS had low ecological risk. Both carcinogenic and non-carcinogenic risk for children and adults (male, female) were within the acceptable range. According to the source analysis. unscientific anthropogenic activities including accumulated MSW, industrial discharges, and vehicle emissions significantly contributed 51.83% to soil trace element contamination. Considering that Tibet is an environment-ecologically vulnerable region with very weak self-adjustment ability, accumulated municipal solid waste in the landfill sites should be well disposed of, and even soil remediation should be well implemented. (C) 2020 Elsevier B.V. All rights reserved.
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页数:11
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