Packed Bed Ca-Cu Looping Process Integrated with a Natural Gas Combined Cycle for Low Emission Power Production

被引:4
|
作者
Martini, Michela [1 ]
Martinez, Isabel [2 ]
Gallucci, Fausto [1 ]
Romano, Matteo C. [2 ]
Chiesa, Paolo [2 ]
Annaland, Martin van Sint [1 ]
机构
[1] Eindhoven Univ Technol, Groene Loper 5, Eindhoven, Netherlands
[2] Politecn Milan, Dept Energy, Via Lambruschini 4, Milan, Italy
关键词
Power production; Chemical looping; Modeling; Sorption enhanced reforming; CO2; capture; CA/CU CHEMICAL LOOP; HYDROGEN-PRODUCTION; CO2; CAPTURE;
D O I
10.1016/j.egypro.2017.03.1153
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This work investigates the full process design of a natural gas combined cycle integrated with a packed-bed reactor system where a hydrogen rich gas is produced with inherent CO2 capture based of the CaO/CaCO3 and Cu/CuO chemical loops. The different stages of this Ca-Cu process were modelled with a dynamic 1D pseudo-homogeneous model, proposing a novel reactor configuration allowing to achieve carbon capture efficiency close to 90%. Process simulations of the whole power plant resulted in electric efficiencies of around 48%(LHV) and SPECCA of 4.7 MJ/kg(CO2). (c) 2017 The Authors. Published by Elsevier Ltd.
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页码:104 / 112
页数:9
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