Theory of valence-band and core-level photoemission from plutonium dioxide

被引：1

作者：

Kolorenc, Jindrich ^{[1
]}

Kozub, Agnieszka L. ^{[1
,2
]}

Shick, Alexander B. ^{[1
]}

机构：

[1] Acad Sci Czech Republ, Inst Phys, Prague 18221, Czech Republic

[2] Gdansk Univ Technol, Fac Appl Phys & Math, PL-80233 Gdansk, Poland

来源：

INTERNATIONAL CONFERENCE ON STRONGLY CORRELATED ELECTRON SYSTEMS 2014 (SCES2014) | 2015年 / 592卷

关键词：

ELECTRONIC-STRUCTURE; ELEMENTS; LIMIT;

D O I：

10.1088/1742-6596/592/1/012054

中图分类号：

O64 [物理化学（理论化学）、化学物理学]; O56 [分子物理学、原子物理学];

学科分类号：

070203 ; 070304 ; 081704 ; 1406 ;

摘要：

The correlated-band theory implemented as a combination of the local-density approximation with the dynamical mean-field theory is applied to PuO2. An insulating electronic structure, consistent with the experimental valence-band photoemission spectra, is obtained. The calculations yield a nonmagnetic ground state that is characterized by a noninteger filling of the plutonium 5f shell. The noninteger filling as well as the satellites appearing in the 4f core-level photoemission spectra originate in a sizable hybridization of the 5f shell with the 2p states of oxygen.

引用

页数：6

共 50 条

[41] DIMER STRUCTURE OF THE SI(001)2 X-1 AND C(4 X-2) RECONSTRUCTIONS DERIVED FROM CORE-LEVEL AND VALENCE-BAND PHOTOEMISSION RESULTS
LANDEMARK, E
KARLSSON, CJ
CHAO, YC
UHRBERG, RIG
SURFACE SCIENCE, 1993, 287 : 529 - 533
[42] VALENCE-BAND AND CORE-LEVEL PHOTOEMISSION-STUDY OF SINGLE-CRYSTAL BI2CASR2CU2O8 SUPERCONDUCTORS
SHEN, ZX
LINDBERG, PAP
WELLS, BO
MITZI, DB
LINDAU, I
SPICER, WE
KAPITULNIK, A
PHYSICAL REVIEW B, 1988, 38 (16): : 11820 - 11823
[43] CAN PHOTOEMISSION MEASURE VALENCE-BAND DISCONTINUITIES
LIST, RS
SPICER, WE
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B, 1988, 6 (04): : 1228 - 1233
[44] Linear dichroism in 3d core-level and 4f valence-band photoemission spectra of strongly correlated rare-earth compounds
Kanai, Y.
Mori, T.
Naimen, S.
Yamagami, K.
Kitayama, S.
Fujiwara, H.
Higashiya, A.
Kadono, T.
Imada, S.
Kiss, T.
Tanaka, A.
Muro, T.
Tamasaku, K.
Yabashi, M.
Ishikawa, T.
Iga, F.
Ebihara, T.
Honda, F.
Onuki, Y.
Sekiyama, A.
JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA, 2017, 220 : 61 - 65
[45] X-RAY PHOTOEMISSION CORE LEVEL DETERMINATION OF THE GASB ALSB HETEROJUNCTION VALENCE-BAND DISCONTINUITY - COMMENT
LEY, L
APPLIED PHYSICS LETTERS, 1987, 50 (24) : 1763 - 1763
[46] Nonequilibrium electronic and phonon dynamics of Cu0.17Bi2Se3 investigated by core-level and valence-band time-resolved photoemission spectroscopy
Yamamoto, T.
Ishida, Y.
Yoshida, R.
Okawa, M.
Okazaki, K.
Kanai, T.
Kikkawa, A.
Taguchi, Y.
Kiss, T.
Ishizaka, K.
Ishii, N.
Itatani, J.
Watanabe, S.
Tokura, Y.
Saitoh, T.
Shin, S.
PHYSICAL REVIEW B, 2015, 92 (12):
[47] VALENCE-BAND AND CU 2P CORE-LEVEL ELECTRONIC-STRUCTURES OF ND2-XCEXCUO4 STUDIED BY X-RAY PHOTOEMISSION
FUKUDA, Y
SUZUKI, T
NAGOSHI, M
SYONO, Y
OHISHI, K
TACHIKI, M
SOLID STATE COMMUNICATIONS, 1989, 72 (12) : 1183 - 1186
[48] Bi ultra-thin crystalline films on InAs(111)A and B substrates: a combined core-level and valence-band angle-resolved and dichroic photoemission study
Nicolai, L.
Mariot, J-M
Djukic, U.
Wang, W.
Heckmann, O.
Richter, M. C.
Kanski, J.
Leandersson, M.
Balasubramanian, T.
Sadowski, J.
Braun, J.
Ebert, H.
Vobornik, I.
Fujii, J.
Minar, J.
Hricovini, K.
NEW JOURNAL OF PHYSICS, 2019, 21 (12):
[49] A NOVEL SOFT-X-RAY SOURCE (H-NU=151.6EV) FOR CORE-LEVEL AND VALENCE-BAND PHOTOEMISSION SPECTROSCOPY WITH HIGH SURFACE SENSITIVITY
DUO, L
DEMICHELIS, B
FASANA, A
ABBATI, I
BRAICOVICH, L
JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA, 1993, 62 (04) : 309 - 316
[50] CORROSION-INHIBITOR SURFACE-CHEMISTRY STUDIED BY CORE AND VALENCE-BAND PHOTOEMISSION
SHERWOOD, PMA
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A-VACUUM SURFACES AND FILMS, 1993, 11 (04): : 2280 - 2285

← 1 2 3 4 5 →