Numerical modeling of a single channel polymer electrolyte fuel cell

被引:5
|
作者
Vasileiadis, N.
Brett, D. J. L.
Vesovic, V.
Kucernak, A. R.
Fontes, E.
Brandon, N. P. [1 ]
机构
[1] Univ London Imperial Coll Sci Technol & Med, Dept Chem Engn, London SW7 2AZ, England
[2] Univ London Imperial Coll Sci Technol & Med, Dept Earth Sci & Engn, London SW7 2AZ, England
[3] Univ London Imperial Coll Sci Technol & Med, Dept Chem, London SW7 2AZ, England
[4] Comsol Ab, Stockholm, Sweden
来源
JOURNAL OF FUEL CELL SCIENCE AND TECHNOLOGY | 2007年 / 4卷 / 03期
基金
英国工程与自然科学研究理事会;
关键词
D O I
10.1115/1.2756557
中图分类号
O646 [电化学、电解、磁化学];
学科分类号
081704 ;
摘要
A two-dimensional model of a single-channel polymer fuel cell has been developed. To achieve model validation, current mapping experiments were performed on the cathode side of a single-channel polymer electrolyte fuel cell (PEFC) of various channel widths, at different reactant flow rates and over a range of operating cell voltages. The fuel side was operated in cross-flow mode, with a high stoichiometric excess of hydrogen to ensure no limitations in anode performance as a function of position along the channel. The solution domain comprises seven regions, (two inlet channels, two diffusers, two active catalyst layers, and a membrane) and considers transport of hydrogen and water vapor in the anode and oxygen and nitrogen and water vapor in the cathode. The resulting set of coupled differential equations was solved numerically with FEMLAB((R)), a MATLAB((R))-based soft ware. The model has been compared to data from a single-channel PEFC, and good agreement between experiment and theory was obtained.
引用
收藏
页码:336 / 344
页数:9
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