Coupling of Carbon Monoxide with Nitrogen Monoxide at a Frustrated Lewis Pair Template

被引：24

作者：

Ye, Ke-Yin ^{[1
]}

Kehr, Gerald ^{[1
]}

Daniliuc, Constantin G. ^{[1
]}

Liu, Lei ^{[2
]}

Grimme, Stefan ^{[2
]}

Erker, Gerhard ^{[1
]}

机构：

[1] Univ Munster, Organ Chem Inst, Corrensstr 40, D-48149 Munster, Germany

[2] Univ Bonn, Inst Phys & Theoret Chem, Mulliken Ctr Theoret Chem, Beringstr 4, D-53115 Bonn, Germany

来源：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2016年 / 55卷 / 32期

基金：

欧洲研究理事会;

关键词：

boron; carbon monoxide; frustrated Lewis pairs; nitric oxide; phosphorus; NITRIC-OXIDE; NITROXYL HNO; BASIS-SETS; CHEMISTRY; ACCURATE; DESIGN;

D O I：

10.1002/anie.201603760

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Coupling of carbon monoxide with nitrogen monoxide was achieved at a frustrated Lewis pair template. This unique reaction uses hydride as an auxiliary, which reductively activates carbon monoxide at the frustrated Lewis pair. The CO/NO coupling reaction then takes place through a pathway involving a radical reaction in which the hydrogen atom auxiliary is eventually removed again.

引用

页码：9216 / 9219

页数：4

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