New insight on the hydrogen bonding structures of nanoconfined water: a Raman study

被引：61

作者：

Crupi, Vincenza ^{[1
]}

Interdonato, Salvatore ^{[1
]}

Longo, Francesca ^{[1
]}

Majolino, Domenico ^{[1
]}

Migliardo, Placido ^{[1
]}

Venuti, Valentina ^{[1
]}

机构：

[1] Univ Messina, Dipartimento Fis, I-98166 Messina, Italy

来源：

JOURNAL OF RAMAN SPECTROSCOPY | 2008年 / 39卷 / 02期

关键词：

confined water; polarised Raman scattering; O-H intra-molecular vibrations;

D O I：

10.1002/jrs.1857

中图分类号：

O433 [光谱学];

学科分类号：

0703 ; 070302 ;

摘要：

Water adsorbed in nanoporous silica glass has been investigated by Raman spectroscopy. The analysis was performed as a function of temperature (from +5 to +75 degrees C), pore diameter (25 and 75 angstrom) and by changing the nature of the substrate (from hydrophilic to hydrophobic) in order to understand the role played on the dynamic peculiarities of water arrangements both by the bare geometrical confinement and the specific interaction with surface. The experimental spectra, collected in the intra-molecular O-H stretching vibrational region, have been decomposed into a sum of sub-bands, representing water molecule arrangements with different types of hydrogen bonding. Hence, we gave a quantitative picture of the temperature and confinement effects on the connectivity pattern. Copyright (C) 2007 John Wiley & Sons, Ltd.

引用

页码：244 / 249

页数：6

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