Importance of aerosols and shape of the cloud droplet size distribution for convective clouds and precipitation

被引:16
|
作者
Barthlott, Christian [1 ]
Zarboo, Amirmahdi [1 ]
Matsunobu, Takumi [2 ]
Keil, Christian [2 ]
机构
[1] Karlsruhe Inst Technol KIT, Inst Meteorol & Climate Res, IMK, TRO,Dept Troposphere Res, Karlsruhe, Germany
[2] Ludwig Maximilians Univ Munchen, Meteorol Inst, Munich, Germany
关键词
MICROPHYSICS PARAMETERIZATION; CONDENSATION NUCLEI; PART I; MODEL; BULK; IMPACT; GERMANY; BIN; INVIGORATION; VARIABILITY;
D O I
10.5194/acp-22-2153-2022
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The predictability of deep moist convection is subject to large uncertainties resulting from inaccurate initial and boundary data, the incomplete description of physical processes, or microphysical uncertainties. In this study, we investigate the response of convective clouds and precipitation over central Europe to varying cloud condensation nuclei (CCN) concentrations and different shape parameters of the cloud droplet size distribution (CDSD), both of which are not well constrained by observations. We systematically evaluate the relative impact of these uncertainties in realistic convection-resolving simulations for multiple cases with different synoptic controls using the new icosahedral non-hydrostatic ICON model. The results show a large systematic increase in total cloud water content with increasing CCN concentrations and narrower CDSDs, together with a reduction in the total rain water content. This is related to a suppressed warm-rain formation due to a less efficient collision-coalescence process. It is shown that the evaporation at lower levels is responsible for diminishing these impacts on surface precipitation, which lies between +13 % and -16 % compared to a reference run with continental aerosol assumption. In general, the precipitation response was larger for weakly forced cases. We also find that the overall timing of convection is not sensitive to the microphysical uncertainties applied, indicating that different rain intensities are responsible for changing precipitation totals at the ground. Furthermore, weaker rain intensities in the developing phase of convective clouds can allow for a higher convective instability at later times, which can lead to a turning point with larger rain intensities later on. The existence of such a turning point and its location in time can have a major impact on precipitation totals. In general, we find that an increase in the shape parameter can produce almost as large a variation in precipitation as a CCN increase from maritime to polluted conditions. The narrowing of the CDSD not only decreases the absolute values of autoconversion and accretion but also decreases the relative role of the warm-rain formation in general, independent of the prevailing weather regime. We further find that increasing CCN concentrations reduce the effective radius of cloud droplets in a stronger manner than larger shape parameters. The cloud optical depth, however, reveals a similarly large increase with larger shape parameters when changing the aerosol load from maritime to polluted. By the frequency of updrafts as a function of height, we show a negative aerosol effect on updraft strength, leading to an enervation of deep convection. These findings demonstrate that both the CCN assumptions and the CDSD shape parameter are important for quantitative precipitation forecasting and should be carefully chosen if double-moment schemes are used for modeling aerosol-cloud interactions.
引用
收藏
页码:2153 / 2172
页数:20
相关论文
共 50 条
  • [31] Dependence of accumulated precipitation on cloud drop size distribution
    Curic, Mladjen
    Janc, Dejan
    Veljovic, Katarina
    [J]. THEORETICAL AND APPLIED CLIMATOLOGY, 2010, 102 (3-4) : 471 - 481
  • [32] Dependence of accumulated precipitation on cloud drop size distribution
    Mladjen Ćurić
    Dejan Janc
    Katarina Veljović
    [J]. Theoretical and Applied Climatology, 2010, 102 : 471 - 481
  • [33] Impact of biomass burning aerosols on radiation, clouds, and precipitation over the Amazon: relative importance of aerosol-cloud and aerosol-radiation interactions
    Liu, Lixia
    Cheng, Yafang
    Wang, Siwen
    Wei, Chao
    Poehlker, Mira L.
    Poehlker, Christopher
    Artaxo, Paulo
    Shrivastava, Manish
    Andreae, Meinrat O.
    Poeschl, Ulrich
    Su, Hang
    [J]. ATMOSPHERIC CHEMISTRY AND PHYSICS, 2020, 20 (21) : 13283 - 13301
  • [34] The effects of aerosols on precipitation and dimensions of subtropical clouds: a sensitivity study using a numerical cloud model
    Teller, A
    Levin, Z
    [J]. ATMOSPHERIC CHEMISTRY AND PHYSICS, 2006, 6 : 67 - 80
  • [35] Quantifying the aerosol effect on droplet size distribution at cloud top
    Pardo, Lianet Hernandez
    Toledo Machado, Luiz Augusto
    Cecchini, Micael Amore
    Gacita, Madeleine Sanchez
    [J]. ATMOSPHERIC CHEMISTRY AND PHYSICS, 2019, 19 (11) : 7839 - 7857
  • [36] Analytical expression for the relative dispersion of the cloud droplet size distribution
    Liu, YG
    Daum, PH
    Yum, SS
    [J]. GEOPHYSICAL RESEARCH LETTERS, 2006, 33 (02)
  • [37] Unsupervised Clustering of Geostationary Satellite Cloud Properties for Estimating Precipitation Probabilities of Tropical Convective Clouds
    Kim, Doyi
    Kim, Hee-jae
    Choi, Yong-sang
    [J]. JOURNAL OF APPLIED METEOROLOGY AND CLIMATOLOGY, 2023, 62 (08) : 1083 - 1094
  • [38] DROPLET SIZE MEASUREMENTS WITH AN OPTICAL CLOUD PARTICLE SPECTROMETER IN NATURAL CLOUDS ON MOUNT WASHINGTON
    HOWE, JB
    GOSSELIN, GA
    [J]. BULLETIN OF THE AMERICAN METEOROLOGICAL SOCIETY, 1976, 57 (02) : 274 - 274
  • [39] Sensitivity of cloud albedo to aerosol concentration and spectral dispersion of cloud droplet size distribution
    Iorga, G.
    Stefan, S.
    [J]. ATMOSFERA, 2007, 20 (03): : 247 - 269
  • [40] MICROSTRUCTURE OF CUMULUS CLOUD .5. CHANGES IN DROPLET SIZE DISTRIBUTION WITH CLOUD AGE
    WARNER, J
    [J]. JOURNAL OF THE ATMOSPHERIC SCIENCES, 1973, 30 (08) : 1724 - 1726