Black carbon in surface soil of the Himalayas and Tibetan Plateau and its contribution to total black carbon deposition at glacial region

被引:15
|
作者
Gautam, Sangita [1 ,2 ]
Yan, Fangping [3 ]
Kang, Shichang [2 ,4 ,5 ]
Han, Xiaowen [1 ,2 ]
Neupane, Bigyan [2 ,4 ]
Chen, Pengfei [4 ]
Hu, Zhaofu [2 ,4 ]
Sillanpaa, Mika [3 ]
Li, Chaoliu [1 ,5 ]
机构
[1] Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing 100101, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[3] LUT Univ, Dept Green Chem, Sammonkatu 12, Mikkeli 50130, Finland
[4] Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Cryospher Sci, Lanzhou 730000, Peoples R China
[5] Chinese Acad Sci, CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100085, Peoples R China
关键词
Black carbon; Mineral dust; Total organic carbon; Surface soil; Glacier; The Himalayas and Tibetan Plateau; LIGHT-ABSORBING IMPURITIES; ORGANIC-CARBON; AEROSOL; ALBEDO; PM2.5; PM10; POLLUTION; INSIGHTS; ELEMENTS; CHARCOAL;
D O I
10.1007/s11356-019-07121-7
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
At present, the glaciers in the Himalayas and the Tibetan Plateau (HTP) are retreating partly due to albedo reduction caused by deposited light-absorbing impurities such as mineral dust (MD) and black carbon (BC). Because BC also exists widely in MD from surface soil, it is necessary to further evaluate the contribution of BC from MD to the total BC at glacier region. This will help to improve the study of BC sources by considering the relative contributions from MD and direct combustion sources. Therefore, in this study, concentrations of total organic carbon (TOC) and fine particles of BC from 43 surface soil samples of the HTP were investigated. The contribution of BC from MD to total BC deposited at the glacier region was evaluated. The results showed strong correlations between TOC and BC of studied samples (R-2 = 0.70, p < 0.01), suggesting that they have similar sources and activity characteristics. The average BC concentration of studied samples was 2.02 +/- 1.55 mg g(-1), much lower than those of particles deposited at the glacier region and other regions with high soil TOC concentration. The contributions of BC from MD to total surface BC at two glaciers of the inner HTP (Zhadang and Xiaodongkemadi) were 17.66 +/- 10.84% and 20.70 +/- 16.35%, respectively. Therefore, the contribution of MD to glacier melting of the HTP is higher than that of previously assumed after BC coming along with MD is considered. Because MD concentration is higher at north and west part of the HTP, the contributions of MD at these glacier regions should be larger than previously assumed.
引用
收藏
页码:2670 / 2676
页数:7
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