Set-up for broadband Fourier-transform multidimensional electronic spectroscopy

被引:14
|
作者
Al Haddad, A. [1 ]
Chauvet, A. [1 ]
Ojeda, J. [1 ]
Arrell, C. [1 ]
van Mourik, F. [1 ]
Auboeck, G. [1 ]
Chergui, M. [1 ]
机构
[1] Ecole Polytech Fed Lausanne, Lab Spectroscopie Ultrarapide, ISIC FSB, CH-1015 Lausanne, Switzerland
关键词
LASER-PULSES; HOLLOW-FIBER; FILAMENTATION; GENERATION; INTENSE;
D O I
10.1364/OL.40.000312
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We present a compact passively phase-stabilized ultra-broadband 2D Fourier transform setup. A gas (argon)-filled hollow core fiber pumped by an amplified Ti:Al2O3 laser is used as a light source providing spectral range spanning from 420 to 900 nm. Sub-10-fs pulses were obtained using a deformable mirror-based pulse shaper. We probe the nonlinear response of Rhodamine 101 using 90 nm bandwidth and resolve vibrational coherences of 150 fs period in the ground state. (C) 2015 Optical Society of America
引用
收藏
页码:312 / 315
页数:4
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