An air-liquid contactor for large-scale capture of CO2 from air

被引:129
|
作者
Holmes, Geoffrey [1 ]
Keith, David W. [1 ,2 ,3 ]
机构
[1] Carbon Engn Ltd, Calgary, AB T2N 1N4, Canada
[2] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA
[3] Harvard Univ, Kennedy Sch Govt, Cambridge, MA 02138 USA
关键词
air capture; carbon dioxide removal; cost optimization; CARBON-DIOXIDE; PROCESS DESIGN; SODIUM;
D O I
10.1098/rsta.2012.0137
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
We present a conceptually simple method for optimizing the design of a gas-liquid contactor for capture of carbon dioxide from ambient air, or 'air capture'. We apply the method to a slab geometry contactor that uses components, design and fabrication methods derived from cooling towers. We use mass transfer data appropriate for capture using a strong NaOH solution, combined with engineering and cost data derived from engineering studies performed by Carbon Engineering Ltd, and find that the total costs for air contacting alone-no regeneration-can be of the order of $60 per tonne CO2. We analyse the reasons why our cost estimate diverges from that of other recent reports and conclude that the divergence arises from fundamental design choices rather than from differences in costing methodology. Finally, we review the technology risks and conclude that they can be readily addressed by prototype testing.
引用
收藏
页码:4380 / 4403
页数:24
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