Single Defect Light-Emitting Diode in a van der Waals Heterostructure

被引:110
|
作者
Clark, Genevieve [1 ]
Schaibley, John R. [2 ]
Ross, Jason [1 ]
Taniguchi, Takashi [3 ]
Watanabe, Kenji [3 ]
Hendrickson, Joshua R. [4 ]
Mou, Shin [5 ]
Yao, Wang [6 ,7 ]
Xu, Xiaodong [1 ,2 ]
机构
[1] Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA
[2] Univ Washington, Dept Phys, Seattle, WA 98195 USA
[3] Natl Inst Mat Sci, Adv Mat Lab, Tsukuba, Ibaraki 3050044, Japan
[4] Air Force Res Lab, Sensors Directorate, Wright Patterson AFB, OH 45433 USA
[5] Air Force Res Lab, Mat & Mfg Directorate, Wright Patterson AFB, OH 45433 USA
[6] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China
[7] Univ Hong Kong, Ctr Theoret & Computat Phys, Hong Kong, Hong Kong, Peoples R China
关键词
Transition metal dichalcogenides; tungsten diselenide; van der Waals heterostructure; electroluminescence; single defect; ATOMICALLY THIN SEMICONDUCTOR; MONOLAYER WSE2; QUANTUM EMITTERS; EMISSION; EXCITONS; DOTS;
D O I
10.1021/acs.nanolett.6b01580
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Single defects in monolayer WSe2 have been shown to be a new class of single photon emitters and have potential applications in quantum technologies. Whereas previous work relied on optical excitation of single defects in isolated WSe2 monolayers, in this work we demonstrate electrically driven single defect light emission by using both vertical and lateral van der Waals heterostructure devices. In both device geometries, we use few layer graphene as the source and drain and hexagonal boron nitride as the dielectric spacer layers for engineered tunneling contacts. In addition, the lateral devices utilize a split back gate design to realize an electrostatically defined p-i-n junction. At low current densities and low temperatures (similar to 5 K), we observe narrow spectral lines in the electroluminescence (EL) whose properties are consistent with optically excited defect bound excitons. We show that the, emission originates from spatially localized regions of the sample, and the EL spectrum from single defects has a doublet with the characteristic exchange splitting and linearly polarized selection rules. All are consistent with previously reported single photon emitters in optical measurements. Our results pave the way for on-chip and electrically driven single photon sources in two-dimensional semiconductors for quantum technology applications.
引用
收藏
页码:3944 / 3948
页数:5
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