Significant emission reductions of carbonaceous aerosols from residential coal burning by a novel stove

被引:1
|
作者
Li, Xuran [1 ,2 ]
Zhang, Chenglong [1 ,2 ,3 ]
Zhuo, Weimin [4 ]
Zhuo, Yuxuan [4 ]
Yang, Jincheng [4 ]
Song, Min [5 ]
Mu, Yujing [1 ,2 ,3 ]
机构
[1] Chinese Acad Sci, Res Ctr Eco Environm Sci, Beijing 100085, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[3] Chinese Acad Sci, Ctr Excellence Urban Atmospher Environm, Inst Urban Environm, Xiamen 361021, Peoples R China
[4] Xuzhou Zhongkai Mech & Elect Equipment Mfg Co Ltd, Xuzhou 221300, Jiangsu, Peoples R China
[5] Shandong Univ, Sch Environm Sci & Engn, Jinan 250100, Peoples R China
基金
中国国家自然科学基金;
关键词
OC; EC; WSOC; Emission factor; Light absorption; POLYCYCLIC AROMATIC-HYDROCARBONS; SOLUBLE ORGANIC-CARBON; LIGHT-ABSORPTION PROPERTIES; BROWN CARBON; ELEMENTAL CARBON; WATER; COMBUSTION; PARTICLES; EXTRACTS; CHINA;
D O I
10.1016/j.jes.2021.08.042
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Carbonaceous aerosols (CA) are crucial components in the atmospheric PM 2.5 and derived from diverse sources. One of the major sources for CA is from the incomplete combustion of bituminous coal that has been prevailingly used by household stoves in rural areas for heating during winter. To efficiently eliminate the CA emission, a new household stove (NHS) was developed based on a novel combustion technology and CA emissions from the NHS and a traditional household stove (THS) were comparably investigated under the actual stove operation conditions in a farmer???s house. Compared with the THS, the emission factors of organic carbon (OC), elemental carbon (EC), and water-soluble organic carbon (WSOC) from the NHS were reduced by 96% ??1%, 98% ??1%, and 91% ??1% under the flaming process and 95% ??1%, 96% ??2%, and 83% ??4% under the smoldering process, respectively. Additionally, the mass absorption efficiency of WSOC from the NHS reduced by 3 folds and the radiative forcing by WSOC relative to EC shrank remarkably by a factor of 3-8. Based on the reduction of emissions and light absorption of WSOC, the promotion of the NHS offers a possible solution to achieve the clean combustion of residential solid fuel. ?? 2022 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.
引用
收藏
页码:135 / 143
页数:9
相关论文
共 50 条
  • [21] Characterizing carbonaceous aerosols in residential coal combustion: Insights from thermal/spectral carbon analyzer coupled with photoionization mass spectrometry analysis
    Jia, Bin
    Zhang, Zhenqiang
    Huang, Zijun
    Feng, Yinchang
    Dai, Qili
    Wu, Fuliang
    Tian, Yingze
    Wu, Jianhui
    [J]. SCIENCE OF THE TOTAL ENVIRONMENT, 2024, 934
  • [22] Effects of Moisture Contents in the Common Oak on Carbonaceous Aerosols Generated from Combustion Processes in an Indoor Wood Stove
    Magnone, Edoardo
    Park, Seong-Kyu
    Park, Jung Hoon
    [J]. COMBUSTION SCIENCE AND TECHNOLOGY, 2016, 188 (06) : 982 - 996
  • [23] Geochemical characteristics and socioeconomic associations of carbonaceous aerosols in coal-fueled cities with significant seasonal pollution pattern
    Xie, Fei
    Guo, Linhao
    Wang, Zichun
    Tian, Yongli
    Yue, Caiying
    Zhou, Xingjun
    Wang, Wei
    Xin, Jinyuan
    Lue, Changwei
    [J]. ENVIRONMENT INTERNATIONAL, 2023, 179
  • [24] Emission characteristics of carbonaceous components and water-soluble ions in PM2.5 from residential coal combustion
    Li, Peng
    Zhou, Wei-Qing
    Xu, Qi-Chun
    Ning, Liang
    Wu, Hua-Cheng
    Zhou, Zi-Long
    Ding, Li-Ping
    [J]. Zhongguo Huanjing Kexue/China Environmental Science, 2022, 42 (11): : 5047 - 5054
  • [25] Modelling carbonaceous aerosol from residential solid fuel burning with different assumptions for emissions
    Ots, Riinu
    Heal, Mathew R.
    Young, Dominique E.
    Williams, Leah R.
    Allan, James D.
    Nemitz, Eiko
    Di Marco, Chiara
    Detournay, Anais
    Xu, Lu
    Ng, Nga L.
    Coe, Hugh
    Herndon, Scott C.
    Mackenzie, Ian A.
    Green, David C.
    Kuenen, Jeroen J. P.
    Reis, Stefan
    Vieno, Massimo
    [J]. ATMOSPHERIC CHEMISTRY AND PHYSICS, 2018, 18 (07) : 4497 - 4518
  • [26] Emission of trace gases and aerosols from biomass burning - an updated assessment
    Andreae, Meinrat O.
    [J]. ATMOSPHERIC CHEMISTRY AND PHYSICS, 2019, 19 (13) : 8523 - 8546
  • [27] Characterization of coal burning-derived individual particles emitted from an experimental domestic stove
    Cong Hou
    Longyi Shao
    Chengmei Zhao
    Jing Wang
    Junxia Liu
    Chunmei Geng
    [J]. Journal of Environmental Sciences, 2018, (09) : 45 - 55
  • [28] Characterization of coal burning-derived individual particles emitted from an experimental domestic stove
    Hou, Cong
    Shao, Longyi
    Zhao, Chengmei
    Wang, Jing
    Liu, Junxia
    Geng, Chunmei
    [J]. JOURNAL OF ENVIRONMENTAL SCIENCES, 2018, 71 : 45 - 55
  • [29] Characterization and emission factors of carbonaceous aerosols originating from coke production in China
    Mu, Ling
    Li, Xuemei
    Liu, Xiaofeng
    Bai, Huiling
    Peng, Lin
    Li, Yangyong
    Tian, Mei
    Zheng, Lirong
    [J]. ENVIRONMENTAL POLLUTION, 2021, 268
  • [30] Wintertime organic aerosols in Christchurch and Auckland, New Zealand: Contributions of residential wood and coal burning and petroleum utilization
    Wang, Haobo
    Kawamura, Kimitaka
    Shooter, David
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2006, 40 (17) : 5257 - 5262