Significant emission reductions of carbonaceous aerosols from residential coal burning by a novel stove

被引:1
|
作者
Li, Xuran [1 ,2 ]
Zhang, Chenglong [1 ,2 ,3 ]
Zhuo, Weimin [4 ]
Zhuo, Yuxuan [4 ]
Yang, Jincheng [4 ]
Song, Min [5 ]
Mu, Yujing [1 ,2 ,3 ]
机构
[1] Chinese Acad Sci, Res Ctr Eco Environm Sci, Beijing 100085, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[3] Chinese Acad Sci, Ctr Excellence Urban Atmospher Environm, Inst Urban Environm, Xiamen 361021, Peoples R China
[4] Xuzhou Zhongkai Mech & Elect Equipment Mfg Co Ltd, Xuzhou 221300, Jiangsu, Peoples R China
[5] Shandong Univ, Sch Environm Sci & Engn, Jinan 250100, Peoples R China
基金
中国国家自然科学基金;
关键词
OC; EC; WSOC; Emission factor; Light absorption; POLYCYCLIC AROMATIC-HYDROCARBONS; SOLUBLE ORGANIC-CARBON; LIGHT-ABSORPTION PROPERTIES; BROWN CARBON; ELEMENTAL CARBON; WATER; COMBUSTION; PARTICLES; EXTRACTS; CHINA;
D O I
10.1016/j.jes.2021.08.042
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Carbonaceous aerosols (CA) are crucial components in the atmospheric PM 2.5 and derived from diverse sources. One of the major sources for CA is from the incomplete combustion of bituminous coal that has been prevailingly used by household stoves in rural areas for heating during winter. To efficiently eliminate the CA emission, a new household stove (NHS) was developed based on a novel combustion technology and CA emissions from the NHS and a traditional household stove (THS) were comparably investigated under the actual stove operation conditions in a farmer???s house. Compared with the THS, the emission factors of organic carbon (OC), elemental carbon (EC), and water-soluble organic carbon (WSOC) from the NHS were reduced by 96% ??1%, 98% ??1%, and 91% ??1% under the flaming process and 95% ??1%, 96% ??2%, and 83% ??4% under the smoldering process, respectively. Additionally, the mass absorption efficiency of WSOC from the NHS reduced by 3 folds and the radiative forcing by WSOC relative to EC shrank remarkably by a factor of 3-8. Based on the reduction of emissions and light absorption of WSOC, the promotion of the NHS offers a possible solution to achieve the clean combustion of residential solid fuel. ?? 2022 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.
引用
收藏
页码:135 / 143
页数:9
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