Facile room-temperature synthesis of highly air-stable and moisture-resistant CsPbX3/SiO2 nanocomposites for tunable white light-emitting diodes

被引:7
|
作者
Chao, Li-Wei [1 ]
Tang, Jian-Fu [1 ]
Lin, Shih-Hung [2 ]
Lee, Yi-Ting [3 ]
Chen, Yi-Lun [4 ,5 ]
Hsieh, Cheng-Ho [4 ,5 ]
Chen, Lung-Chien [1 ]
Tseng, Zong-Liang [4 ,5 ]
机构
[1] Natl Taipei Univ Technol, Dept Electroopt Engn, 1,Sec 3,Chung Hsiao E Rd, Taipei 106, Taiwan
[2] Natl Yunlin Univ Sci & Technol, Dept Elect Engn, Touliu 64002, Yunlin, Taiwan
[3] Kyushu Univ, Ctr Organ Photon & Elect Res OPERA, 744 Motooka, Nishi, Fukuoka 8190395, Japan
[4] Ming Chi Univ Technol, Dept Elect Engn, 84 Gungjuan Rd, New Taipei 24301, Taiwan
[5] Ming Chi Univ Technol, Organ Elect Res Ctr, 84 Gungjuan Rd, New Taipei 24301, Taiwan
关键词
Perovskite QDs; SiO2; Stability; White LED; WIDE COLOR GAMUT; PEROVSKITE QUANTUM DOTS; ANION-EXCHANGE; HIGH-STABILITY; LEDS; NANOCRYSTALS; EFFICIENCY;
D O I
10.1016/j.mssp.2021.106158
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
All inorganic perovskite quantum dots (PQDs) and perovskite CsPbX3/SiO2 nanocomposites (PNCs) have shown their potentials for optical and lighting applications. We demonstrate a one-step approach to synthesize PQDs and PNCs more simply and effectively at room temperature in the open air. The resulting PNCs can show a narrow emission in the PL spectra and high stability under ambient conditions. In particular, both green CsPbBr3/SiO2 and red CsPbI3-xBrx/SiO2 PNCs can be obtained by employing this easy and low-cost method. Even, the SiO2 protection can also effectively prevent the halide exchange reaction between green and red PNCs, meaning the capability for white light applications. The resulting white light-emitting diodes (WLEDs) based on the green and red PNCs coated on the blue LED have a white Commission Internationale del' Enclairage (CIE) coordinates of (0.375, 0.362) and a low correlated color temperature (CCT) of 4054 K.
引用
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页数:7
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