Geometric Design of Anode-Supported Micro-Tubular Solid Oxide Fuel Cells by Multiphysics Simulations

被引:3
|
作者
Shi, Hong-yu
Zhu, Jiang
Lin, Zi-jing [1 ]
机构
[1] Univ Sci & Technol China, Dept Phys, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China
基金
中国国家自然科学基金;
关键词
I-V relations; Thermal fluid electrochemistry model; Parametric optimization; Volumetric power density; Anode thickness; MASS-TRANSPORT; SOFC STACK; FABRICATION; MICROSTRUCTURE; PERFORMANCE; ISSUES;
D O I
10.1063/1674-0068/30/cjcp1704071
中图分类号
O64 [物理化学(理论化学)、化学物理学]; O56 [分子物理学、原子物理学];
学科分类号
070203 ; 070304 ; 081704 ; 1406 ;
摘要
High volumetric power density (VPD) is the basis for the commercial success of micro-tubular solid oxide fuel cells (mtSOFCs). To find maximal VPD (MVPD) for anode-supported mtSOFC (as-mtSOFC), the effects of geometric parameters on VPD are analyzed and the anode thickness, t(an), and the cathode length, l(ca), are identified as the key design parameters. Thermo-fluid electrochemical models were built to examine the dependence of the electrical output on the cell parameters. The multiphysics model is validated by reproducing the experimental I-V curves with no adjustable parameters. The optimal l(ca) and the corresponding MVPDs are then determined by the multiphysics model for 20 combinations of r(in), the inner tube radius, and t(an). And all these optimization are made at 1073.15 K. The results show that: (i) significant performance improvement may be achieved by geometry optimization, (ii) the seemingly high MVPD of 11 and 14 W/cm(3) can be easily realized for as-mtSOFC with single-and double-terminal anode current collection, respectively. Moreover, the variation of the area specific power density with l(ca) is an element of(2 mm, 40 mm) is determined for three representative (r(in), t(an)) combinations. Besides, it is demonstrated that the current output of mtSOFC with proper geometric parameters is comparable to that of planar SOFC.
引用
收藏
页码:411 / 417
页数:7
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