Solid state 31P and 207Pb MAS NMR studies on polycrystalline 0,0′-dialkyldithiophosphate lead(II) complexes

被引：35

作者：

Larsson, AC

Ivanov, AV

Pike, KJ

Forsling, W

Antzutkin, ON ^{[1
]}

机构：

[1] Univ Lulea, Div Chem, S-97187 Lulea, Sweden

[2] Russian Acad Sci, Far Eastern Branch, Amur Integrated Res Inst, Blagoveshchensk 675000, Russia

[3] ANSTO, Mat & Engn Sci, Lucas Heights, NSW 2234, Australia

来源：

JOURNAL OF MAGNETIC RESONANCE | 2005年 / 177卷 / 01期

关键词：

P-31; CP/MAS; (207) Pb MAS NMR; P-31 chemical shift anisotropy; (207) Pb chemical shift anisotropy; 0,0 '-dialkyldithiophosphate lead(II) complexes; (2)J(P-31; (207); Pb)-coupling;

D O I：

10.1016/j.jmr.2005.07.007

中图分类号：

Q5 [生物化学];

学科分类号：

071010 ; 081704 ;

摘要：

A number of lead(II) O,O'-dialkyldithiophosphate complexes were studied by C-13, P-31, and Pb-207 MAS NMR. Simulations of P-31 chemical shift anisotropy using spinning sideband analysis reveal a linear relationship between the S-P-S bond angle and the principal values delta(22) and delta(33) of the P-31 chemical shift tensor. The P-31 CSA data were used to assign ligands with different structural functions. In the cases of diethyldithiophosphate and di-iso-butyldithiophosphate lead(II) complexes, (2)J(P-31, Pb-207)-couplings were resolved and used to confirm the suggested assignment of the ligands. The SIMPSON computer program was used to calculate P-31 and Pb-207 spectral sideband patterns. (c) 2005 Elsevier Inc. All rights reserved.

引用

下载

页码：56 / 66

页数：11

共 50 条

[41] Characterising Lone-Pair Activity of Lead(II) by 207Pb Solid-State NMR Spectroscopy: Coordination Polymers of [N(CN)2]- and [Au(CN)2]- with Terpyridine Ancillary Ligands
Greer, Brandon J.
Michaelis, Vladimir K.
Katz, Michael J.
Leznoff, Daniel B.
Schreckenbach, Georg
Kroeker, Scott
CHEMISTRY-A EUROPEAN JOURNAL, 2011, 17 (13) : 3609 - 3618
[42] Solid state 14N and 31P MAS NMR:: New tools to study electrostatic binding of peptides on biomembrane surfaces.
Lindström, F
Sani, M
Williamson, PTF
Bokvist, M
Gröbner, G
BIOPHYSICAL JOURNAL, 2004, 86 (01) : 19A - 19A
[43] Hydronium Ions on the Surface of a Partially Hydrolyzed α-Zirconium Phosphate: Solid-State 2H and 31P MAS NMR Evidence
Bakhmutov, Vladimir, I
Drake, Hannah F.
Zhou, Hong-Cai
INORGANIC CHEMISTRY, 2022, 61 (18) : 6715 - 6719
[44] 31P solid-state NMR studies of the short-range order in phosphorus-selenium glasses
Bytchkov, Aleksei
Fayon, Franck
Massiot, Dominique
Hennet, Louis
Price, David L.
PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2010, 12 (07) : 1535 - 1542
[45] NMR studies of 31P, 1H spin pairs in solid tin(II) phosphite and tin(II) hydrogen phosphate
Amornsakchai, P
Hodgkinson, P
Harris, RK
MOLECULAR PHYSICS, 2004, 102 (9-10) : 877 - 882
[46] P-31, PT-195 AND PB-207 NMR-STUDIES ON SOME PLATINUM-LEAD BONDED COMPOUNDS
CARR, S
COLTON, R
DAKTERNIEKS, D
JOURNAL OF ORGANOMETALLIC CHEMISTRY, 1982, 240 (02) : 143 - 151
[47] Solid-state 31P and 109Ag CP/MAS NMR as a powerful tool for studying of silver(I) complexes with N-thiophosphorylated thiourea and thioamide ligands
Rakhmatullin, Aydar
Brusko, Vasiliy V.
Shcherbitskaya, Elmira R.
Polovov, Ilya B.
Bakirov, Rinat
Bessada, Catherine
MAGNETIC RESONANCE IN CHEMISTRY, 2022, 60 (09) : 893 - 900
[48] Complexation of lead(II) with O,O′-dialkyldithlophosphate ligands:: 31P and 13C CP/MAS NMR and single-crystal X-ray diffraction studies
Larsson, AC
Ivanov, AV
Antzutkin, ON
Gerasimenko, AV
Forsling, W
INORGANICA CHIMICA ACTA, 2004, 357 (09) : 2510 - 2518
[49] 15N and 31P solid-state NMR investigations on the orientation of zervamicin II and alamethicin in phosphatidylcholine membranes
Bechinger, B
Skladnev, DA
Ogrel, A
Li, X
Rogozhkina, EV
Ovchinnikova, TV
O'Neil, JDJ
Raap, J
BIOCHEMISTRY, 2001, 40 (31) : 9428 - 9437
[50] Influence of the CaO/MgO ratio on the structure of phase-separated glasses:: a solid state 29Si and 31P MAS NMR study
Oliveira, JM
Correia, RN
Fernandez, MH
Rocha, J
JOURNAL OF NON-CRYSTALLINE SOLIDS, 2000, 265 (03) : 221 - 229

← 1 2 3 4 5 →