Motional effect in surface sum-frequency vibrational spectroscopy

被引：149
|
作者：
Wei, X [1 ]
Shen, YR
机构：
[1] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
[2] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA
来源：
PHYSICAL REVIEW LETTERS | 2001年 / 86卷 / 21期
关键词：
D O I：
10.1103/PhysRevLett.86.4799
中图分类号：
O4 [物理学];
学科分类号：
0702 ;
摘要：
Fast orientational motion of molecules at a surface can affect the sum-frequency vibrational spectra of the surface. Calculation shows that the effect is significant if the molecular orientation varies over a broad range within the vibrational relaxation time. The stretch vibration of the free OH bonds at the vapor/water interface ib used to illustrate the importance of the effect.
引用
收藏
页码：4799 / 4802
页数：4
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