Synthesis gas production process for natural gas conversion over Ni-La2O3 catalyst

被引:8
|
作者
Cho, Wonjun [1 ]
Yu, Hyejin [1 ,2 ]
Ahn, Wha-Seung [2 ]
Kim, Seung-Soo [3 ]
机构
[1] KOGAS, DME Technol Res Ctr, Inchon 406130, South Korea
[2] Inha Univ, Dept Chem Engn, Inchon 402751, South Korea
[3] Kangwon Natl Univ, Dept Chem Engn, Samcheok 245711, Gangwon Do, South Korea
关键词
Syngas; Steam-CO2 reforming (SCR); Synthetic fuel reactor; Catalyst; Kinetics; METHANE; CO2; CHALLENGES; REACTOR; COKE;
D O I
10.1016/j.jiec.2015.02.019
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The synthesis gas (syngas) is a mixture of hydrogen and carbon monoxide, which is suitable as a feed gas to produce clean liquid synthetic fuel in natural gas conversion reactor. In order to achieve the efficiency reactor, the syngas composition should match the usage ratio of the reactors. In this work, we investigate the development of synthesis gas production process in the steam-CO2 reforming (SCR) over Ni-La2O3 catalyst supported Ce-ZrO2/Al2O3. And, we developed the kinetics model for SCR used by the profiles of concentration and temperature in the SCR reactor. (C) 2015 The Korean Society of Industrial and Engineering Chemistry. Published by Elsevier B.V. All rights reserved.
引用
收藏
页码:229 / 235
页数:7
相关论文
共 50 条
  • [31] Hydrogen production by steam reforming of liquefied natural gas (LNG) over mesoporous Ni-La-Al2O3 aerogel catalysts: Effect of La content
    Bang, Yongju
    Seo, Jeong Gil
    Song, In Kyu
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2011, 36 (14) : 8307 - 8315
  • [32] Development of synthesis gas production catalyst and process.
    Yagi, F
    Wakamatsu, S
    Kanai, R
    Kajiyama, R
    Suehiro, Y
    Shimura, M
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2004, 228 : U665 - U665
  • [33] Enhanced Investigation of CO Methanation over Ni/Al2O3 Catalysts for Synthetic Natural Gas Production
    Hu, Dacheng
    Gao, Jiajian
    Ping, Yuan
    Jia, Lihua
    Gunawan, Poernomo
    Zhong, Ziyi
    Xu, Guangwen
    Gu, Fangna
    Su, Fabing
    INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2012, 51 (13) : 4875 - 4886
  • [34] Production of CO-rich hydrogen gas from glycerol dry reforming over La-promoted Ni/Al2O3 catalyst
    Siew, Kah Weng
    Lee, Hua Chyn
    Gimbun, Jolius
    Cheng, Chin Kui
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2014, 39 (13) : 6927 - 6936
  • [35] Oxidation behavior of a Ni-La2O3 codeposited film on nickel
    Peng, X
    Ping, DH
    Li, TF
    Wu, WT
    JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1998, 145 (02) : 389 - 398
  • [36] Coupling of exothermic and endothermic reactions in oxidative conversion of natural gas into ethylene/olefins over diluted SrO/La2O3/SA5205 catalyst
    Choudhary, VR
    Mulla, SAR
    INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1997, 36 (09) : 3520 - 3527
  • [37] CO Methanation Toward the Production of Synthetic Natural Gas over Highly Active Ni/TiO2 Catalyst
    Shinde, Vijay M.
    Madras, Giridhar
    AICHE JOURNAL, 2014, 60 (03) : 1027 - 1035
  • [38] Catalytic steam reforming of glycerol over Ni-La2O3-CeO2/SBA-15 catalyst for stable hydrogen-rich gas production
    Moogi, Surendar
    Lee, In-Gu
    Hwang, Kyung-Ran
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2020, 45 (53) : 28462 - 28475
  • [39] Synthesis of N-methylmorpholine over the catalyst Cu-Ni-Co/Al2O3 in the gas phase
    Chen, Han-Geng
    Zhang, Tao
    Luo, Ming
    Qian, Chao
    Liu, Jin-Qiang
    Han, Xiao
    Chen, Xin-Zhi
    Gao Xiao Hua Xue Gong Cheng Xue Bao/Journal of Chemical Engineering of Chinese Universities, 2009, 23 (05): : 801 - 806
  • [40] Catalytic partial oxidation of methane to synthesis gas over Ni/γ-Al2O3 catalyst in a fluidized-bed
    Ji, YY
    Li, WZ
    Xu, HY
    Chen, YX
    APPLIED CATALYSIS A-GENERAL, 2001, 213 (01) : 25 - 31