Dry reforming of methane to hydrogen-rich syngas over robust fibrous KCC-1 stabilized nickel catalyst with high activity and coke resistance
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作者:
Abdulrasheed, A. A.
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Univ Teknol Malaysia, Fac Engn, Sch Chem & Energy Engn, Utm Johor Bahru 81310, Johor, Malaysia
Abubakar Tafawa Balewa Univ, Dept Chem Engn, PMB 0248, Bauchi, Bauchi State, NigeriaUniv Teknol Malaysia, Fac Engn, Sch Chem & Energy Engn, Utm Johor Bahru 81310, Johor, Malaysia
Abdulrasheed, A. A.
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Jalil, A. A.
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Univ Teknol Malaysia, Fac Engn, Sch Chem & Energy Engn, Utm Johor Bahru 81310, Johor, Malaysia
Univ Teknol Malaysia, Ctr Hydrogen Energy, Inst Future Energy, Utm Johor Bahru 81310, Johor, MalaysiaUniv Teknol Malaysia, Fac Engn, Sch Chem & Energy Engn, Utm Johor Bahru 81310, Johor, Malaysia
Jalil, A. A.
[1
,2
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Hamid, M. Y. S.
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Univ Teknol Malaysia, Fac Engn, Sch Chem & Energy Engn, Utm Johor Bahru 81310, Johor, MalaysiaUniv Teknol Malaysia, Fac Engn, Sch Chem & Energy Engn, Utm Johor Bahru 81310, Johor, Malaysia
Hamid, M. Y. S.
[1
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Siang, T. J.
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Univ Teknol Malaysia, Fac Engn, Sch Chem & Energy Engn, Utm Johor Bahru 81310, Johor, MalaysiaUniv Teknol Malaysia, Fac Engn, Sch Chem & Energy Engn, Utm Johor Bahru 81310, Johor, Malaysia
Siang, T. J.
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Fatah, N. A. A.
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Univ Teknol Malaysia, Fac Engn, Sch Chem & Energy Engn, Utm Johor Bahru 81310, Johor, MalaysiaUniv Teknol Malaysia, Fac Engn, Sch Chem & Energy Engn, Utm Johor Bahru 81310, Johor, Malaysia
Fatah, N. A. A.
[1
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Izan, S. M.
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Univ Teknol Malaysia, Fac Sci, Dept Chem, Utm Johor Bahru 81310, Johor, MalaysiaUniv Teknol Malaysia, Fac Engn, Sch Chem & Energy Engn, Utm Johor Bahru 81310, Johor, Malaysia
Izan, S. M.
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Hassan, N. S.
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Univ Teknol Malaysia, Fac Engn, Sch Chem & Energy Engn, Utm Johor Bahru 81310, Johor, MalaysiaUniv Teknol Malaysia, Fac Engn, Sch Chem & Energy Engn, Utm Johor Bahru 81310, Johor, Malaysia
Hassan, N. S.
[1
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机构:
[1] Univ Teknol Malaysia, Fac Engn, Sch Chem & Energy Engn, Utm Johor Bahru 81310, Johor, Malaysia
[2] Univ Teknol Malaysia, Ctr Hydrogen Energy, Inst Future Energy, Utm Johor Bahru 81310, Johor, Malaysia
[3] Univ Teknol Malaysia, Fac Sci, Dept Chem, Utm Johor Bahru 81310, Johor, Malaysia
A remarkably stable and active nickel (Ni) catalyst, supported on fibrous KCC-1 silica particles, was prepared by in situ one-pot hydrothermal method to produce a hydrogenrich syngas. The catalysts' properties were characterized by BET, XRD, FESEM-mapping, FTIR-pyrrole, FTIR-KBr, and XPS, while coke deposition was evaluated using Raman spectra, TEM and TGA/DTA. The high dispersion of Ni crystallites, enhanced basicity, strong Ni-KCC-1 interaction, and encapsulation of Ni particles contributed to the enhanced catalyst stability and activity. The one-pot catalyst produced high CH4 and CO2 conversions at 92% and 88% respectively, with high H-2/CO ratio, and an extended stability over 72 h at 750 degrees C. There was limited coke deposition, predominantly of the amorphous type, owing to its synthesis method and support morphology. (C) 2019 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.