Air quality and emissions in the Yangtze River Delta, China

被引:136
|
作者
Li, L. [1 ]
Chen, C. H. [1 ]
Fu, J. S. [2 ]
Huang, C. [1 ]
Streets, D. G. [3 ]
Huang, H. Y. [1 ]
Zhang, G. F. [1 ]
Wang, Y. J. [4 ]
Jang, C. J. [5 ]
Wang, H. L. [1 ]
Chen, Y. R. [1 ]
Fu, J. M. [4 ]
机构
[1] Shanghai Acad Environm Sci, Shanghai 200233, Peoples R China
[2] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA
[3] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA
[4] Shanghai Univ, Sch Environm & Chem Engn, Inst Environm Pollut & Hlth, Shanghai 200444, Peoples R China
[5] US EPA, Off Air Qual Planning & Stand, Res Triangle Pk, NC 27711 USA
关键词
MODELING SYSTEM; EAST-ASIA; OZONE POLLUTION; GASEOUS-POLLUTANTS; BOUNDARY-LAYER; RURAL SITE; SHANGHAI; SO2; NOX; SENSITIVITY;
D O I
10.5194/acp-11-1621-2011
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Regional trans-boundary air pollution has become an important issue in the field of air pollution modeling. This paper presents the results of the implementation of the MM5-CMAQ modeling system in the Yangtze River Delta (YRD) for the months of January and July of 2004. The meteorological parameters are obtained by using the MM5 model. A new regional emission inventory with spatial and temporal allocations based on local statistical data has been developed to provide input emissions data to the MM5-CMAQ modeling system. The pollutant concentrations obtained from the MM5-CMAQ modeling system have been compared with observational data from the national air pollution monitoring network. It is found that air quality in winter in the YRD is generally worse than in summer, due mainly to unfavorable meteorological dispersion conditions. In winter, the pollution transport from Northern China to the YRD reinforces the pollution caused by large local emissions. The monthly average concentration of SO2 in the YRD is 0.026 +/- 0.011 mg m(-3) in January and 0.017 +/- 0.009 mg m(-3) in July. Monthly average concentrations of NO2 in the YRD in January and July are 0.021 +/- 0.009 mg m(-3), and 0.014 +/- 0.008 mg m(-3), respectively. The monthly average concentration of PM10 in the YRD is 0.080 +/- 0.028 mg m(-3) in January and 0.025 +/- 0.015 mg m(-3) in July. Visibility is also a problem, with average deciview values of 26.4 +/- 2.95 dcv in winter and 17.6 +/- 3.3 dcv in summer. The ozone concentration in the downtown area of a city like Zhoushan can be very high, with the highest simulated value reaching 0.24 mg m(-3). In January, the monthly average concentration of O-3 in the YRD is 0.052 +/- 0.011 mg m(-3), and 0.054 +/- 0.008 mg m(-3) in July. Our results show that ozone and haze have become extremely important issues in the regional air quality. Thus, regional air pollution control is urgently needed to improve air quality in the YRD.
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页码:1621 / 1639
页数:19
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