Fundamental understanding of the acidic oxygen evolution reaction: mechanism study and state-of-the-art catalysts

被引：216

作者：

Shi, Zhaoping ^{[1
,2
]}

Wang, Xian ^{[2
,3
,4
]}

Ge, Junjie ^{[2
,3
,4
]}

Liu, Changpeng ^{[2
,3
,4
]}

Xing, Wei ^{[1
,2
]}

机构：

[1] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Electroanalyt Chem, Changchun 130022, Jilin, Peoples R China

[2] Univ Sci & Technol China, Hefei 230026, Anhui, Peoples R China

[3] Chinese Acad Sci, Changchun Inst Appl Chem, Lab Adv Power Sources, Changchun 130022, Jilin, Peoples R China

[4] Jilin Prov Key Lab Low Carbon Chem Power Sources, Changchun 130022, Jilin, Peoples R China

来源：

NANOSCALE | 2020年 / 12卷 / 25期

基金：

中国国家自然科学基金; 国家重点研发计划;

关键词：

WATER OXIDATION; BIFUNCTIONAL ELECTROCATALYST; ELECTRONIC-STRUCTURE; HIGHLY EFFICIENT; OXIDE-FILMS; DOPED TIO2; ASSISTED SYNTHESIS; LATTICE-STRAIN; ACTIVE-SITES; FUEL-CELL;

D O I：

10.1039/d0nr02410d

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The oxygen evolution reaction (OER), as the anodic reaction of water electrolysis (WE), suffers greatly from low reaction kinetics and thereby hampers the large-scale application of WE. Seeking active, stable, and cost-effective OER catalysts in acidic media is therefore of great significance. In this perspective, studying the reaction mechanism and exploiting advanced anode catalysts are of equal importance, where the former provides guidance for material structural engineering towards a better catalytic activity. In this review, we first summarize the currently proposed OER catalytic mechanisms,i.e., the adsorbate evolution mechanism (AEM) and lattice oxygen evolution reaction (LOER). Subsequently, we critically review several acidic OER electrocatalysts reported recently, with focus on structure-performance correlation. Finally, a few suggestions on exploring future OER catalysts are proposed.

引用

页码：13249 / 13275

页数：27

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