Probing Transient Localized Electromagnetic Fields Using Low- Energy Point-Projection Electron Microscopy

被引:11
|
作者
Hergert, Germann [1 ,2 ]
Woeste, Andreas [1 ,2 ]
Vogelsang, Jan [1 ,2 ]
Quenzel, Thomas [1 ,2 ]
Wang, Dong [3 ,4 ]
Gross, Petra [1 ,2 ]
Lienau, Christoph [1 ,2 ,5 ]
机构
[1] Carl von Ossietzky Univ Oldenburg, Inst Phys, D-26129 Oldenburg, Germany
[2] Carl von Ossietzky Univ Oldenburg, Ctr Interface Sci, D-26129 Oldenburg, Germany
[3] TU Ilmenau, Inst Werkstofftech, D-98693 Ilmenau, Germany
[4] TU Ilmenau, Inst Mikro & Nanotechnol MakroNano, D-98693 Ilmenau, Germany
[5] Carl von Ossietzky Univ Oldenburg, Forschungszentrum Neurosensor, D-26129 Oldenburg, Germany
关键词
ultrafast electron microscopy; streaking spectroscopy; point-projection electron microscopy; surface plasmon polaritons; adiabatic nanofocusing; charge dynamics; OPTICAL-EXCITATIONS; DRIVEN;
D O I
10.1021/acsphotonics.1c00775
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Low kinetic energy electrons are of interest for probing nanoscale dynamic processes using ultrafast electron microscopy techniques. Their low velocities reduce radiation doses and enhance the interaction with confined electromagnetic fields and, thus, may enable ultrafast spectroscopy of single nanostructures. Recent improvements in the spatial and temporal resolution of ultrafast, low-energy electron microscopy have been achieved by combining nanotip photoemitters and point-projection imaging schemes. Here, we use such an ultrafast point-projection electron microscope (UPEM) to analyze the interaction of low-energy electrons with transient electric fields created by photoemission from a nanogap antenna. By analyzing their kinetic energy distribution, we separate angular deflection due to radial field components from electron energy gain and loss due to their axial acceleration. Our measurements open up a route toward the spatial and temporal characterization of vectorial near-fields by low energy electron streaking spectroscopy.
引用
收藏
页码:2573 / 2580
页数:8
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