Biochemical composite synthesized by stepwise crosslinking: An efficient platform for one-pot biomass conversion

被引：9

作者：

Wei, Wei ^{[1
,2
]}

Wang, Cong ^{[1
,2
]}

Zhao, Yu ^{[1
,2
]}

Peng, Shichao ^{[1
,2
]}

Zhang, Haoyang ^{[1
,2
]}

Bian, Yipeng ^{[1
,2
]}

Li, Hexing ^{[1
,2
]}

Zhou, Xinggui ^{[3
]}

Li, Hui ^{[1
,2
]}

机构：

[1] Shanghai Normal Univ, Educ Minist, Key Lab Resource Chem, Shanghai 200234, Peoples R China

[2] Shanghai Normal Univ, Shanghai Key Lab Rare Earth Funct Mat, Shanghai 200234, Peoples R China

[3] E China Univ Sci & Technol, State Key Lab Chem Engn, Shanghai 200237, Peoples R China

来源：

JOURNAL OF CATALYSIS | 2015年 / 327卷

基金：

中国国家自然科学基金;

关键词：

Biochemical composite; Yolk-shell nanostructure; Metallic catalysis; Enzymatic catalysis; Biomass conversion; AMORPHOUS ALLOY; GLUCOSE HYDROGENATION; SPHERICAL SILICA; GLUCOAMYLASE; IMMOBILIZATION; ENZYME; SHELL; CATALYST; NICKEL; ROUTES;

D O I：

10.1016/j.jcat.2015.04.021

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

This paper describes the development of a new bifunctional catalyst system that integrates enzyme and chemical material into a biochemical composite through a stepwise crosslinking approach. The as-prepared biochemical composite not only allows "one-pot" biomass conversion via sequential enzyme-catalyzed hydrolysis of biomass materials to glucose and metal-catalyzed hydrogenation of glucose to sorbitol, but also enables reusability of the catalyst. This design concept facilitates access to fuels and chemicals from the biomass-derived sorbitol and will attract more attention in the foreseeable future. (C) 2015 Elsevier Inc. All rights reserved.

引用

页码：78 / 85

页数：8

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