Raman spectra of proton order of thin ice Ih film

被引：17
|
作者：
Men, Zhiwei [1 ]
Fang, Wenhui [2 ]
Wang, Shenghan [1 ]
Li, Zhanlong [1 ]
Sun, Chenglin [1 ,3 ]
Wang, Xiaojun [3 ]
机构：
[1] Jilin Univ, Coll Phys, Changchun 130012, Peoples R China
[2] Changchun Univ Sci & Technol, Sch Sci, Changchun 130022, Peoples R China
[3] Georgia So Univ, Dept Phys, Statesboro, GA 30460 USA
来源：
JOURNAL OF RAMAN SPECTROSCOPY | 2015年 / 46卷 / 04期
关键词：
ice Ih; ice XI; LO-TO splitting; Fermi resonance; FERMI RESONANCE; WATER;
D O I：
10.1002/jrs.4666
中图分类号：
O433 [光谱学];
学科分类号：
0703 ; 070302 ;
摘要：
The polarized Raman spectra of the upper part of a thin ice Ih film were obtained in the range of 150cm(-1) to 3800cm(-1). The spectra showed clear polarization dependence; several new peaks were also observed. The longitudinaloptic-tranverseoptic (LO-TO) splitting of the mode near 220cm(-1) in the translational vibration region was experimentally confirmed at 133K. The Fermi resonance between the bending overtone (around 3270cm(-1)) and symmetry stretching fundamental (around 3350cm(-1)) in the stretching vibration region appeared at nearly the same temperature. Results showed that ice XI (i.e. proton-ordered phase of ice Ih) slowly formed in the upper part of a thin ice Ih film without KOH as the temperature gradually decreased below 133K. Copyright (c) 2015 John Wiley & Sons, Ltd.
引用
收藏
页码：388 / 391
页数：4
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