Emission Reduction of NOx, CO, HC, PM2.5, and PAHs by Using a Catalyst in a Diesel Engine

被引:5
|
作者
Chou, Feng-Chih [1 ,2 ]
Jhang, Syu-Ruei [3 ]
Lin, Sheng-Lun [4 ]
Chen, Chung-Bang [5 ]
Chen, Kang-Shin [1 ,2 ]
Lin, Yuan-Chung [1 ,2 ,6 ]
机构
[1] Natl Sun Yat Sen Univ, Inst Environm Engn, Kaohsiung 804, Taiwan
[2] Natl Sun Yat Sen Univ, Ctr Emerging Contaminants Res, Kaohsiung 804, Taiwan
[3] Acad Sinica, Res Ctr Environm Changes, Taipei 11529, Taiwan
[4] Beijing Inst Technol, Sch Mech Engn, Beijing 100081, Peoples R China
[5] CPC Corp, Fuel Qual & Automobile Emiss Res Div, Refining & Mfg Res Inst, Chiayi 600, Taiwan
[6] Kaohsiung Med Univ, Coll Hlth Sci, Dept Publ Hlth, Kaohsiung 807, Taiwan
关键词
Diesel engine; EGP-SCR; PM2.5; PAHs; Lifetime carcinogenic risk; POLYCYCLIC AROMATIC-HYDROCARBONS; PARTICLE-SIZE DISTRIBUTION; AIR-POLLUTANTS; DIBENZOFURANS; BIODIESEL; OPERATION; VEHICLES; EXHAUSTS; DUST;
D O I
10.4209/aaqr.220180
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Pollutants derived from diesel exhaust gases are considered harmful to human health. In 2021, 23 million motor vehicles were in use, and diesel cars accounted for 4.07% of them. Strategies involving after-treatment technologies, with exhaust gas processing incorporating a selective catalytic reaction (EGP-SCR system) for diesel engines, are considered in this study. By conducting a World Harmonized Transient Cycle (WHTC) under cold start driving test, this study measured pollutant emissions upstream and downstream of the after-treatment system. Our results indicate that equipped with EGP-SCR catalysts as after treatment device can eliminate particles and regulated pollutants from the engine out emissions. LMW g-PAHs (two- and three-ring PAHs) provided the largest contribution to exhaust emissions, accounting for more than 90% of total PAHs. After the EGP-SCR treatment was applied, LMW g-PAHs were identified the highest reduction followed by MMW g-PAHs and HMW g-PAHs. It is noteworthy that, the reduction of p-PAHs was related to the decrease of total particulate matter (PM2.5) when the SCR device was applied, and the reduction rate of 56.7% can be observed. However, low exhaust temperature of the diesel engine leads to the activity of the SCR catalyst being reduced, and it was thus not capable of decomposing PAHs effectively. The ILCR values for g-PAHs were 1.93 x 10(-3) and 1.45 x 10(-3) in adults and children, respectively, indicating potential health risk in this study. The data reveal that the EGP-SCR system can effectively decline regulated and help avoid inhalation of carcinogenic substances (PM2.5). Moreover, g-PAHs create serious carcinogenic hazards, cannot be suppressed by the EGP-SCR after-treatment system under cold start condition.
引用
收藏
页数:15
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