Emission Reduction of NOx, CO, HC, PM2.5, and PAHs by Using a Catalyst in a Diesel Engine

被引:5
|
作者
Chou, Feng-Chih [1 ,2 ]
Jhang, Syu-Ruei [3 ]
Lin, Sheng-Lun [4 ]
Chen, Chung-Bang [5 ]
Chen, Kang-Shin [1 ,2 ]
Lin, Yuan-Chung [1 ,2 ,6 ]
机构
[1] Natl Sun Yat Sen Univ, Inst Environm Engn, Kaohsiung 804, Taiwan
[2] Natl Sun Yat Sen Univ, Ctr Emerging Contaminants Res, Kaohsiung 804, Taiwan
[3] Acad Sinica, Res Ctr Environm Changes, Taipei 11529, Taiwan
[4] Beijing Inst Technol, Sch Mech Engn, Beijing 100081, Peoples R China
[5] CPC Corp, Fuel Qual & Automobile Emiss Res Div, Refining & Mfg Res Inst, Chiayi 600, Taiwan
[6] Kaohsiung Med Univ, Coll Hlth Sci, Dept Publ Hlth, Kaohsiung 807, Taiwan
关键词
Diesel engine; EGP-SCR; PM2.5; PAHs; Lifetime carcinogenic risk; POLYCYCLIC AROMATIC-HYDROCARBONS; PARTICLE-SIZE DISTRIBUTION; AIR-POLLUTANTS; DIBENZOFURANS; BIODIESEL; OPERATION; VEHICLES; EXHAUSTS; DUST;
D O I
10.4209/aaqr.220180
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Pollutants derived from diesel exhaust gases are considered harmful to human health. In 2021, 23 million motor vehicles were in use, and diesel cars accounted for 4.07% of them. Strategies involving after-treatment technologies, with exhaust gas processing incorporating a selective catalytic reaction (EGP-SCR system) for diesel engines, are considered in this study. By conducting a World Harmonized Transient Cycle (WHTC) under cold start driving test, this study measured pollutant emissions upstream and downstream of the after-treatment system. Our results indicate that equipped with EGP-SCR catalysts as after treatment device can eliminate particles and regulated pollutants from the engine out emissions. LMW g-PAHs (two- and three-ring PAHs) provided the largest contribution to exhaust emissions, accounting for more than 90% of total PAHs. After the EGP-SCR treatment was applied, LMW g-PAHs were identified the highest reduction followed by MMW g-PAHs and HMW g-PAHs. It is noteworthy that, the reduction of p-PAHs was related to the decrease of total particulate matter (PM2.5) when the SCR device was applied, and the reduction rate of 56.7% can be observed. However, low exhaust temperature of the diesel engine leads to the activity of the SCR catalyst being reduced, and it was thus not capable of decomposing PAHs effectively. The ILCR values for g-PAHs were 1.93 x 10(-3) and 1.45 x 10(-3) in adults and children, respectively, indicating potential health risk in this study. The data reveal that the EGP-SCR system can effectively decline regulated and help avoid inhalation of carcinogenic substances (PM2.5). Moreover, g-PAHs create serious carcinogenic hazards, cannot be suppressed by the EGP-SCR after-treatment system under cold start condition.
引用
收藏
页数:15
相关论文
共 50 条
  • [1] Plasma PM and NOx treatment for diesel engine emission
    Yamamoto, T.
    Kajimoto, A.
    Yoshida, K.
    Okubo, M.
    Kuroki, T.
    PROGRESS OF GREEN OXIDATION/REDUCTION TECHNOLOGIES, 2006, : 336 - 340
  • [2] Reduction of smoke, PM2.5, and NOx of a diesel engine integrated with methanol steam reformer recovering waste heat and cooled EGR
    Wu, Horng-Wen
    Hsu, Tzu-Ting
    Fan, Chen-Ming
    He, Po-Hsien
    ENERGY CONVERSION AND MANAGEMENT, 2018, 172 : 567 - 578
  • [3] Co-benefits of CO2 and PM2.5 emission reduction
    Yang, Siyuan
    Chen, Bin
    Ulgiati, Sergio
    CLEAN ENERGY FOR CLEAN CITY: CUE 2016 - APPLIED ENERGY SYMPOSIUM AND FORUM: LOW-CARBON CITIES AND URBAN ENERGY SYSTEMS, 2016, 104 : 92 - 97
  • [4] Emissions of PAHs, Nitro-PAHs and Quinones (Oxy-PAHs) Associated to PM1.0 and PM2.5 Emitted by a Diesel Engine Fueled with Diesel-Biodiesel-Ethanol Blends
    Paim, Joilson Nascimento
    Santos, Aldenor Gomes
    Araujo, Rennan G. O.
    Nascimento, Madson Moreira
    De Andrade, Jailson Bittencourt
    Guarieiro, Lilian Lefol Nani
    ATMOSPHERE, 2023, 14 (04)
  • [5] Experimental investigation of HC and CO emission reduction from a diesel engine powered by plastic oil blend using fly ash as catalyst
    S. Premkumar
    G. Balaji
    Journal of Thermal Analysis and Calorimetry, 2022, 147 : 1535 - 1545
  • [6] Experimental investigation of HC and CO emission reduction from a diesel engine powered by plastic oil blend using fly ash as catalyst
    Premkumar, S.
    Balaji, G.
    JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY, 2022, 147 (02) : 1535 - 1545
  • [7] Characterization and quantification of PM2.5 emissions and PAHs concentration in PM2.5 from the exhausts of diesel vehicles with various accumulated mileages
    Lin, Yuan-Chung
    Li, Ya-Ching
    Amesho, Kassian T. T.
    Chou, Feng-Chih
    Cheng, Pei-Cheng
    SCIENCE OF THE TOTAL ENVIRONMENT, 2019, 660 : 188 - 198
  • [8] Significantly mitigating PM2.5 pollution level via reduction of NOx emission during wintertime
    Fu, Shuang
    Liu, Pengfei
    He, Xiaowei
    Song, Yifei
    Liu, Junfeng
    Zhang, Chenglong
    Mu, Yujing
    SCIENCE OF THE TOTAL ENVIRONMENT, 2023, 898
  • [9] PM and NOx removal for diesel engine emission using ozonizer and chemical hybrid reactor
    Yamamoto, Toshiaki
    Kajimoto, Akinori
    Okubo, Masaaki
    Kuroki, Tomoyuki
    Yoshida, Keiichiro
    IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS, 2008, 44 (05) : 1431 - 1435
  • [10] Emission Inventory of Pollutants (CO, SO2, PM2.5, and NOx) In Jakarta Indonesia
    Lestari, Puji
    Damayanti, Seny
    Arrohman, Maulana Khafid
    15TH INTERNATIONAL CONFERENCE ON ATMOSPHERIC SCIENCES AND APPLICATIONS TO AIR QUALITY, 2020, 489