Soil contamination by potentially toxic elements and the associated human health risk in geo- and anthropogenic contaminated soils: A case study from the temperate region (Germany) and the arid region (Egypt)

被引:73
|
作者
Shaheen, Sabry M. [1 ,2 ,3 ]
Antoniadis, Vasileios [4 ]
Kwon, Eilhann [5 ]
Song, Hocheol [5 ]
Wang, Shan-Li [6 ]
Hseu, Zeng-Yei [6 ]
Rinklebe, Joerg [1 ,5 ]
机构
[1] Univ Wuppertal, Sch Architecture & Civil Engn, Lab Soil & Groundwater Management, Pauluskirchstr 7, D-42285 Wuppertal, Germany
[2] King Abdulaziz Univ, Fac Meteorol Environm & Arid Land Agr, Dept Arid Land Agr, Jeddah 21589, Saudi Arabia
[3] Univ Kafrelsheikh, Fac Agr, Dept Soil & Water Sci, Kafr Al Sheikh 33516, Egypt
[4] Univ Thessaly, Dept Agr Crop Prod & Rural Environm, Volos, Greece
[5] Sejong Univ, Dept Environm, Dept Environm & Energy, Seoul 05006, South Korea
[6] Natl Taiwan Univ, Dept Agr Chem, 1 Sect 4,Roosevelt Rd, Taipei 10617, Taiwan
关键词
Soil origin; Toxic metal(loid)s; Risk assessment; Contamination indices; HEAVY-METAL POLLUTION; RARE-EARTH-ELEMENTS; GEOCHEMICAL FRACTIONS; NILE DELTA; PROFILES; RIVER; ZN; CU; SEDIMENTS; PLANT;
D O I
10.1016/j.envpol.2020.114312
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The aim of this study was to assess the soil contamination caused by potentially toxic elements (Al, As, Co, Cr, Cu, Fe, Mn, Mo, Ni, Se, V, and Zn) using various indices and the associated risk of human health for adults and children in selected soils from Germany (Calcic Luvisols, Tidalic Fluvisols, Haplic Gleysols, and Eutric Fluvisols) and Egypt (Haplic Calcisols, Sodic Fluvisols, and Eutric Fluvisols). Soil contamination degree has been assessed using indices such as contamination factor (CF), pollution load index (PLI), geoaccumulation index (Igeo), and enrichment factor. We also assessed the health risk for children and for male and female adults. Chromium, Cu, As, Mo, Ni, Se, and Zn in the German Fluvisols had high CF of >6, while in the Egyptian Fluvisols Se, Mo, As, and Al revealed a high CF. The PLI (1.1-5.2) was higher than unity in most soils (except for Tidalic Fluvisols), while the most important contributor was Se, followed by Mo and As in the Egyptian Fluvisols, and by Cr, Cu, and Zn in the German Fluvisols. The median value of hazard index (HI) for children in the studied soils indicated an elevated health risk (higher than one), especially in the German Fluvisols (HI = 4.0-29.0) and in the Egyptian Fluvisols (HI = 2.2-5.2). For adults, median HIs in all soils were lower than unity for both males and females. The key contributor to HI was As in the whole soil profiles, accounting for about 59% of the total HIs in all three person groupings. Our findings show that in the studied multi-element contaminated soils the risk for children's health is higher than for adults; while mainly As (and Al, Cr, Cu, and Fe) contributed significantly to soil-derived health risk. (C) 2020 Elsevier Ltd. All rights reserved.
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页数:10
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